Abstract
This paper presents the seasonality of vertical profiles of CO2 within 0–1100 m at a suburban site and discussions on the impacts of meteorological parameters on it. CO2 concentrations as well as metrological conditions were measured on June 2–18, July 7–22 (21 days, summer), October 10–20 (10 days, autumn) in 2012, and January 15–February 1 (12 days, winter), May 7–23 (10 days, spring) in 2013. The CO2 vertical profiles were affected by meteorological conditions, source emissions, urban canopy and other factors. The CO2 concentrations’ comparison analysis between different seasons including spring, summer (previously published results), autumn and winter suggests that the highest peak of the CO2 concentration (450.00 ± 14.78 ppm) occurred during winter (2013-01-23 at 09:00–09:55) with neutral stability class whereas the lowest peak of the CO2 concentration (389.88 ± 4.67 ppm) occurred during summer (2012-07-17 at 15:48–16:40) with moderately stable conditions. The high levels of CO2 concentrations were due to the accumulation caused by the stable atmosphere dominant during the measurement period. Atmospheric CO2 concentrations in summer can be lower near the surface than at elevated altitude under certain conditions because terrestrial photosynthesis dominated the industrial pollutant emissions at that time. However, in other seasons, CO2 profiles showed monotonically declining trends with altitudes.
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Adams AM, Prospero JM, Zhang C (2012) Calipso-derived three-dimensional structure of aerosol over the atlantic basin and adjacent continents. J Clim 25(19):6862–6879. https://doi.org/10.1175/JCLI-D-11-00672.1
Barnola JM (1999) Status of the atmospheric CO2 reconstruction from ice cores analyses. Tellus B 51(2):151–155. https://doi.org/10.1034/j.1600-0889.1999.t01-1-00002.x
Bischof W, Fabian P, Borchers R (1980) Decrease in CO2 mixing ratio observed in the stratosphere. Nature 288:347–348. https://doi.org/10.1038/288347a0
Bolton D (1980) The computation of equivalent potential temperature. Mon Weather Rev 108(7):1046–1053. https://doi.org/10.1175/1520-0493(1980)108<1046:tcoept>2.0.co;2
Chen B, Chen JM, Liu J, Chan D, Higuchi K, Shashkov A (2004) A vertical diffusion scheme to estimate the atmospheric rectifier effect. J Geophys Res Atmos 109(D4):D04306. https://doi.org/10.1029/2003JD003925
Davy R, Esau I (2016) Differences in the efficacy of climate forcings explained by variations in atmospheric boundary layer depth. Nat Commun. https://doi.org/10.1038/ncomms11690
Denning AS, Fung IY, Randall D (1995) Latitudinal gradient of atmospheric CO2 due to seasonal exchange with land biota. Nature 376(6537):240–243
Engelen RJ, McNally AP (2005) Estimating atmospheric CO2 from advanced infrared satellite radiances within an operational four-dimensional variational (4d-var) data assimilation system: results and validation. J Geophys Res Atmos 110(D18):D18305. https://doi.org/10.1029/2005JD005982
Esau I, Zilitinkevich S (2010) On the role of the planetary boundary layer depth in the climate system. Adv Sci Res 4:63
Eugster W, Siegrist F (2000) The influence of nocturnal CO2 advection on CO2 flux measurements. Basic Appl Ecol 1(2):177–188. https://doi.org/10.1078/1439-1791-00028
Ferrero L, Riccio A, Perrone MG, Sangiorgi G, Ferrini BS, Bolzacchini E (2011) Mixing height determination by tethered balloon-based particle soundings and modeling simulations. Atmos Res 102(1–2):145–156. https://doi.org/10.1016/j.atmosres.2011.06.016
Garratt JR (1994) The atmospheric boundary layer. Earth-Sci Rev 37(1):89–134. https://doi.org/10.1016/0012-8252(94)90026-4
Guo J, Liu H, Wang F, Huang J, Xia F, Lou M, Wu Y, Jiang JH, Xie T, Zhaxi Y (2016a) Three-dimensional structure of aerosol in china: a perspective from multi-satellite observations. Atmos Res 178:580–589. https://doi.org/10.1016/j.atmosres.2016.05.010
Guo J, Miao Y, Zhang Y, Liu H, Li Z, Zhang W, He J, Lou M, Yan Y, Bian L, Zhai P (2016b) The climatology of planetary boundary layer height in china derived from radiosonde and reanalysis data. Atmos Chem Phys 16(20):13309–13319. https://doi.org/10.5194/acp-16-13309-2016
Gurk C, Fischer H, Hoor P, Lawrence MG, Lelieveld J, Wernli H (2008) Airborne in situ measurements of vertical, seasonal and latitudinal distributions of carbon dioxide over europe. Atmos Chem Phys Discuss 8(2):7315–7337. https://doi.org/10.5194/acpd-8-7315-2008
Huang J, Guo J, Wang F, Liu Z, Jeong MJ, Yu H, Zhang Z (2015) Calipso inferred most probable heights of global dust and smoke layers. J Geophys Res Atmos 120(10):5085–5100. https://doi.org/10.1002/2014JD022898
Lawrence MG (2005) The relationship between relative humidity and the dewpoint temperature in moist air: a simple conversion and applications. Bull Am Meteorol Soc 86(2):225–233. https://doi.org/10.1175/bams-86-2-225
Li Y, Deng J, Mu C, Xing Z, Du K (2014) Vertical distribution of CO2 in the atmospheric boundary layer: characteristics and impact of meteorological variables. Atmos Environ 91:110–117. https://doi.org/10.1016/j.atmosenv.2014.03.067
Machida T, Kita K, Kondo Y, Blake D, Kawakami S, Inoue G, Ogawa T (2002a) Vertical and meridional distributions of the atmospheric CO2 mixing ratio between northern midlatitudes and southern subtropics. J Geophys Res Atmos. https://doi.org/10.1029/2001JD000910
Machida T, Kita K, Kondo Y, Blake D, Kawakami S, Inoue G, Ogawa T (2002b) Vertical and meridional distributions of the atmospheric CO2 mixing ratio between northern midlatitudes and southern subtropics. J Geophys Res Atmos. https://doi.org/10.1029/2001JD000910
Monteith J, Unsworth M (2007) Principles of environmental physics. Academic Press, Cambridge
Murayama S, Saigusa N, Chan D, Yamamoto S, Kondo H, Eguchi Y (2003) Temporal variations of atmospheric CO2 concentration in a temperate deciduous forest in central Japan. Tellus B 55(2):232–243. https://doi.org/10.1034/j.1600-0889.2003.00061.x
Pickett-Heaps CA, Rayner PJ, Law RM, Ciais P, Patra PK, Bousquet P, Peylin P, Maksyutov S, Marshall J, Rödenbeck C, Langenfelds RL, Steele LP, Francey RJ, Tans P, Sweeney C (2011) Atmospheric CO2 inversion validation using vertical profile measurements: analysis of four independent inversion models. J Geophys Res Atmos. https://doi.org/10.1029/2010JD014887
Sangiorgi G, Ferrero L, Perrone MG, Bolzacchini E, Duane M, Larsen BR (2011) Vertical distribution of hydrocarbons in the low troposphere below and above the mixing height: tethered balloon measurements in milan, italy. Environ Pollut 159(12):3545–3552. https://doi.org/10.1016/j.envpol.2011.08.012
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The authors thank the support from the National Natural Science Foundation of China (No. 41005081) and financial supports through University of Calgary Eyes High doctoral recruiting scholarship.
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Esteki, K., Prakash, N., Li, Y. et al. Seasonal Variation of CO2 Vertical Distribution in the Atmospheric Boundary Layer and Impact of Meteorological Parameters. Int J Environ Res 11, 707–721 (2017). https://doi.org/10.1007/s41742-017-0062-y
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DOI: https://doi.org/10.1007/s41742-017-0062-y