Skip to main content
Log in

Reference device for calibration of radon exhalation rate measuring instruments and its performance

  • Published:
Nuclear Science and Techniques Aims and scope Submit manuscript

Abstract

Environmental radon emanates from the exhalation and release of soil, rocks, and building materials. Environmental radon contamination tracing and radon pollution prevention and control require the measurement of the radon exhalation rate on media surfaces. Reliable measurements of the radon exhalation rate cannot be achieved without regular calibration of the measuring instrument with a high-performance reference device. In this study, a reference device for the calibration of radon exhalation rate measuring instruments was developed using a diffusion solid radon source with a high and stable radon emanation coefficient, an integrated diffusion component composed of a plasterboard and a high-density wooden board, an air pressure balance device, a radon accumulation chamber, and a support structure. The uniformity and stability of the reference device were evaluated using the activated carbon-γ spectrum and open-loop method, respectively, to measure the radon exhalation rate. The reference device achieved different radon exhalation rates by using different activities of diffusion solid radon sources. Nineteen measurement points were regularly selected on the radon exhalation surface of the reference device, and the uniformity of the radon exhalation rate exceeded 5%. The short-term stability of the reference device was better than 5% under different environmental conditions and was almost unaffected by the ambient air pressure, environmental temperature, and relative humidity.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6
Fig. 7
Fig. 8
Fig. 9

Similar content being viewed by others

Data availability

The data that support the findings of this study are openly available in Science Data Bank at https://doi.org/10.57760/sciencedb.j00186.00136 and https://cstr.cn/31253.11.sciencedb.j00186.00136.

References

  1. N. Lavi, V. Steiner, Z.B. Alfassi, Measurement of radon emanation in construction materials. Radiat. Meas. 44(4), 396–400 (2009). https://doi.org/10.1016/j.radmeas.2009.04.009

    Article  Google Scholar 

  2. United Nations Scientific Committee on the Effects of Atomic Radiation. Effects of Ionizing Radiation, United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) 2006 Report, Volume I: Report to the General Assembly, Scientific Annexes A and B. United Nations, 2008. https://doi.org/10.18356/7fb405cb-en

  3. D.-K. Ting, WHO handbook on indoor radon: a public health perspective. Int. J. Environ. Stud. 67(1), 100–102 (2010). https://doi.org/10.1080/00207230903556771

    Article  Google Scholar 

  4. Y. Huo, P. Xu, C. Zhou et al., Effect of environment humidity to radon measurement with SSNTD. Nucl. Sci. Tech. 20(4), 228–230 (2009). https://doi.org/10.13538/j.1001-8042/nst.20.228-230

    Article  Google Scholar 

  5. J. Somlai, Z. Gorjánácz, A. Várhegyi et al., Radon concentration in houses over a closed Hungarian uranium mine. Sci. Total Environ. 367(2–3), 653–665 (2006)

    Article  ADS  Google Scholar 

  6. J. Jónás, J. Somlai, E. Tóth-Bodrogi et al., Study of a remediated coal ash depository from a radiological perspective. J. Environ. Radioactiv. 173, 75–84 (2017). https://doi.org/10.1016/j.jenvrad.2016.11.010

    Article  Google Scholar 

  7. X.J. Li, S.K. Qiu, C.K. Liu, A calibration facility for radon fluxmeter. Radiat. Prot. 28(4), 197–201 (2008). (in Chinese)

    Google Scholar 

  8. S. Röttger, A. Röttger, C. Grossi et al., Radon metrology for use in climate change observation and radiation protection at the environmental level. Adv. Geosci. 57, 37–47 (2022). https://doi.org/10.5194/adgeo-57-37-2022

    Article  Google Scholar 

  9. P.Y. Wang, Y.F. Jia, Reduce indoor pollution and share fresh air—interpretation of GB 50325–2020 “Standard for door Environmental Pollution Control of Civil Building Engineering.” Constr. Qual. 39(03), 1–5 (2021). (in Chinese)

    Google Scholar 

  10. L.D. Lv, Z.Z. He, S.K. Qiu et al., Evaluation and measurement methods for the surface radon exhalation rate of buildings. Indoor Built Environ. 31(10), 2378–2385 (2022). https://doi.org/10.1177/1420326X221109754

    Article  Google Scholar 

  11. Y.F. Yang, L.D. Lv, S.K. Qiu et al., Study on the influence of sampling methods for measuring soil radon exhalation rates. Radiat. Meas. 159, 106880 (2022). https://doi.org/10.1016/j.radmeas.2022.106880

    Article  Google Scholar 

  12. GB/T(Chinese Standards) GB/T 16143-1995. Charcoal canister method for measuring 222Rn exhalation rate from building surface (English Vision). Beijing: National Health Commission of the People’s Republic of China, 1995.

  13. Y.L. Tan, D.T. Xiao, H. Yuan et al., Revision for measuring radon exhalation rate in open loop. J. Instrum. 8(01), T01004 (2013). https://doi.org/10.1088/1748-0221/8/01/T01004

    Article  Google Scholar 

  14. J.N. Hartley, G.W. Gee, E.G. Baker, et al., 1981 Radon barrier field test at Grand Junction uranium mill tailings pile. Pacific Northwest Lab. Richland, WA (USA), 1983. https://www.osti.gov/biblio/6405607

  15. R. Collé, J.M.R. Hutchinson, M.P. Unterweger, The NIST primary radon-222 measurement system. J. Res. Natl. Inst. Stan. 95(2), 155 (1990). https://doi.org/10.6028/jres.095.018

    Article  Google Scholar 

  16. L.D. Lv, X.P. Qiu, S.K. Qiu et al., Study of active carbon measuring method for accurate measurements of radon exhalation rates for building materials. J. Univ. South China (Sci. Technol.) 28(01), 9–12 (2014). https://doi.org/10.19431/j.cnki.1673-0062.2014.01.004 (in Chinese)

    Article  ADS  Google Scholar 

  17. A. Tsapalov, K. Kovler, P. Miklyav, Open charcoal chamber method for mass measurements of radon exhalation rate from soil surface. J. Environ. Radioactiv. 160, 28–35 (2016). https://doi.org/10.1016/j.jenvrad.2016.04.016

    Article  Google Scholar 

  18. X.S. Liu, S.K. Qiu, A rapid and accurate method for measuring radon exhalation rate. Radiat. Prot. 27(03), 156–162 (2007). https://doi.org/10.3321/j.issn:1000-8187.2007.03.005 (in Chinese)

    Article  Google Scholar 

  19. Q. Tang, S.K. Qiu, D.T. Xiao et al., Extraction and purification of 227Ac and development of solid 219Rn source. Radiochim. Acta 102(1–2), 169–174 (2014). https://doi.org/10.1515/ract-2014-2117

    Article  Google Scholar 

  20. J. Ke, Y.L. Ke, Y.H. Zhuang et al., The analysis of the performance in the calibration of radon measurement instrument by several kinds of solid standard source. South China J. Seismol. 35(2), 43–49 (2015). https://doi.org/10.13512/j.hndz.2015.02.007 (in Chinese)

    Article  Google Scholar 

  21. W.Y. Du, GD—L2 Flow-type solid radon source calibration factors of radon measurement instrument and its influence. J. Inst. Disaster Prev. 15(3), 67–71 (2013). https://doi.org/10.3969/j.issn.1673-8047.2013.03.012 (in Chinese)

    Article  MathSciNet  Google Scholar 

  22. E. Saleh, A.M.A. Al-Sobahi, S.A.E. El-Fiki, Assessment of radon exhalation rate, radon concentration and annual effective dose of some building materials samples used in Yemen. Acta Geophys. 69(4), 1325–1333 (2021). https://doi.org/10.1007/s11600-021-00628-z

    Article  ADS  Google Scholar 

  23. M. Noguchi, H. Wakita, A method for continuous measurement of radon in groundwater for earthquake prediction. J. Geophys. Res. 82(8), 1353–1357 (1977). https://doi.org/10.1029/JB082i008p01353

    Article  ADS  Google Scholar 

  24. H.N.P. Thu, N. Van Thang, L.C. Hao, The effects of some soil characteristics on radon emanation and diffusion. J. Environ. Radioactiv. 216, 106189 (2020). https://doi.org/10.1016/j.jenvrad.2020.106189

    Article  Google Scholar 

  25. C. Miró, E. Andrade, M. Reis et al., Development of a couple of methods for measuring radon exhalation from building materials commonly used in the Iberian Peninsula. Radiat. Prot. Dosim. 160(1–3), 177–180 (2014). https://doi.org/10.1093/rpd/ncu063

    Article  Google Scholar 

  26. Z.Q. Li, D.T. Xiao, G.Z. Zhao et al., Rapid determination of radon monitor’s calibration factors. Nucl. Sci. Tech. 27, 116 (2016). https://doi.org/10.1007/s41365-016-0118-2

    Article  Google Scholar 

  27. P. Tuccimei, M. Moroni, D. Norcia, Simultaneous determination of 222Rn and 220Rn exhalation rates from building materials used in Central Italy with accumulation chambers and a continuous solid state alpha detector: influence of particle size, humidity and precursors concentration. Appl. Radiat. Isot. 64(2), 254–263 (2006). https://doi.org/10.1016/j.apradiso.2005.07.016

    Article  Google Scholar 

  28. G.P. Xiao, D.T. Xiao, L.D. Lv et al., Study on active carbon sampling device for measuring radon exhalation rate. Nucl. Electron. Detect. Technol. 35(11), 1119–1123 (2015). https://doi.org/10.3969/j.issn.0258-0934.2015.11.016 (in Chinese)

    Article  Google Scholar 

  29. C.E. Lawrence, R.A. Akber, A. Bollhöfer et al., Radon-222 exhalation from open ground on and around a uranium mine in the wet-dry tropics. J. Environ. Radioact. 100(1), 1–8 (2009). https://doi.org/10.1016/j.jenvrad.2008.09.003

    Article  Google Scholar 

  30. S.H. Alharbi, R.A. Akber, Radon-222 activity flux measurement using activated charcoal canisters: revisiting the methodology. J. Environ. Radioact. 129, 94–99 (2014). https://doi.org/10.1016/j.jenvrad.2013.12.021

    Article  Google Scholar 

  31. J.L. Pinault, J.C. Baubron, Signal processing of diurnal and semidiurnal variations in radon and atmospheric pressure: a new tool for accurate in situ measurement of soil gas velocity, pressure gradient, and tortuosity. J. Geophys. Res. Solid Earth 102(B8), 18101–18120 (1997). https://doi.org/10.1029/97JB00971

    Article  Google Scholar 

Download references

Acknowledgements

We are particularly grateful to Drs. Shao-Bin Guan, Zong-Jie Zhou, Feng-Lin Li, and Tao Sun of the Chinese Nuclear Industry Remote Sensing Center for providing support under experimental conditions.

Author information

Authors and Affiliations

Authors

Contributions

All authors contributed to the study conception and design. Material preparation, data collection and analysis were performed by Wei-Gang Li, De-Tao Xiao, Zheng-Zhong He, Xiang-Yuan Deng and Shou-Kang Qiu. The first draft of the manuscript was written by Wei-Gang Li and all authors commented on previous versions of the manuscript. All authors read and approved the final manuscript.

Corresponding author

Correspondence to De-Tao Xiao.

Ethics declarations

Conflict of interest

The authors declare that they have no conflict of interest.

Additional information

This work was supported by the National Natural Science Foundation of China (No.11875165).

Rights and permissions

Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Li, WG., Xiao, DT., He, ZZ. et al. Reference device for calibration of radon exhalation rate measuring instruments and its performance. NUCL SCI TECH 34, 128 (2023). https://doi.org/10.1007/s41365-023-01275-3

Download citation

  • Received:

  • Revised:

  • Accepted:

  • Published:

  • DOI: https://doi.org/10.1007/s41365-023-01275-3

Keywords

Navigation