Abstract
The enhanced surface plasmon (SP) coupling effects in a blue light-emitting diode (LED) with regularly patterned (REG) surface Ag nanoparticles (NPs) on a dielectric interlayer (DI) of a lower refractive index overgrown on p-GaN are demonstrated. Without a DI, the surface Ag NPs-induced SP coupling with the quantum wells (QWs) in the LED can lead to the increases of internal quantum efficiency and LED output intensity, the reduction of the external quantum efficiency droop effect, and the enhancement of modulation response. By adding a DI, the SP coupling effect is enhanced, resulting in the further improvements of all the aforementioned factors. We compare the SP coupling effects in the LEDs with REG Ag NPs on DIs to those of randomly distributed (RAN) Ag NPs previously reported. Although the variation trends of the localized surface plasmon (LSP) resonance peaks and hence the SP coupling behaviors of REG and RAN Ag NPs are similar, their LSP resonance strengths at the QW emission wavelength are different due to their different spectral patterns of LSP resonance. In other words, although the REG Ag NPs can produce stronger collective LSP resonance with a narrower spectral width, the SP coupling effect depends mainly on the LSP resonance strength at the QW emission wavelength.
Similar content being viewed by others
References
Yeh DM, Huang CF, Chen CY, Lu YC, Yang CC (2007) Surface plasmon coupling effect in an InGaN/GaN single-quantum-well light-emitting diode. Appl Phys Lett 91(17):171103
Sun G, Khurgin JB, Soref RA (2007) Practicable enhancement of spontaneous emission using surface plasmons. Appl Phys Lett 90(11):111107
Shen KC, Chen CY, Chen HL, Huang CF, Kiang YW, Yang CC, Yang YJ (2008) Enhanced and partially polarized output of a light-emitting diode with Its InGaN/GaN quantum well coupled with surface plasmons on a metal grating. Appl Phys Lett 93(23):231111
Kwon MK, Kim JY, Kim BH, Park IK, Cho CY, Byeon CC, Park SJ (2008) Surface-plasmon-enhanced light-emitting diodes. Adv Mater 20(7):1253–1257
Lin J, Mohammadizia A, Neogi A, Morkoç H, Ohtsu M (2010) Surface plasmon enhanced UV emission in AlGaN/GaN quantum well. Appl Phys Lett 97(22):221104
Kuo Y, Ting SY, Liao CH, Huang JJ, Chen CY, Hsieh C, Lu YC, Chen CY, Shen KC, Lu CF, Yeh DM, Wang JY, Chuang WH, Kiang YW, Yang CC (2011) Surface plasmon coupling with radiating dipole for enhancing the emission efficiency of a light-emitting diode. Opt Express 19(S4):A914–A929
Cho CY, Lee SJ, Song JH, Hong SH, Lee SM, Cho YH, Park SJ (2011) Enhanced optical output power of green light-emitting diodes by surface plasmon of gold nanoparticles. Appl Phys Lett 98(5):051106
N. Gao, K. Huang, J. Li, S. Li, X. Yang, and J. Kang (2012) Surface-plasmon-enhanced deep-UV light emitting diodes based on AlGaN multi-quantum wells, Scientific Reports 2(#816), 00816
Chen HS, Chen CF, Kuo Y, Chou WH, Shen CH, Jung YL, Kiang YW, Yang CC (2013) Surface plasmon coupled light-emitting diode with metal protrusions into p-GaN. Appl Phys Lett 102(4):041108
Cho CY, Zhang Y, Cicek E, Rahnema B, Bai Y, McClintock R, Razeghi M (2013) Surface plasmon enhanced light emission from AlGaN-based ultraviolet light-emitting diodes grown on Si (111). Appl Phys Lett 102(21):211110
Schubert MF, Xu J, Kim JK, Schubert EF, Kim MH, Yoon S, Lee SM, Sone C, Sakong T, Park Y (2008) Polarization-matched GaInN/AlGaInN multi-quantum-well light-emitting diodes with reduced efficiency droop. Appl Phys Lett 93(4):041102
Xie J, Ni X, Fan Q, Shimada R, Özgür Ü, Morkoç H (2008) On the efficiency droop in InGaN multiple quantum well blue light emitting diodes and its reduction with p-doped quantum well barriers. Appl Phys Lett 93(12):121107
Maier M, Köhler K, Kunzer M, Pletschen W, Wagner J (2009) Reduced nonthermal rollover of wide-well GaInN light-emitting diodes. Appl Phys Lett 94(4):041103
Delaney KT, Rinke P, Van de Walle CG (2009) Auger recombination rates in nitrides from first principles. Appl Phys Lett 94(19):191109
Kioupakis E, Rinke P, Delaney KT, Van de Walle CG (2011) Indirect Auger recombination as a cause of efficiency droop in nitride light-emitting diodes. Appl Phys Lett 98(16):161107
Iveland J, Martinelli L, Peretti J, Speck JS, Weisbuch C (2013) Direct measurement of Auger electrons emitted from a semiconductor light-emitting diode under electrical injection: identification of the dominant mechanism for efficiency droop. Phys Rev Lett 110(17):177406
Lu CF, Liao CH, Chen CY, Hsieh C, Kiang YW, Yang CC (2010) Reduction of the efficiency droop effect of a light-emitting diode through surface plasmon coupling. Appl Phys Lett 96(26):261104
Lin CH, Hsieh C, Tu CG, Kuo Y, Chen HS, Shih PY, Liao CH, Kiang YW, Yang CC, Lai CH, He GR, Yeh JH, Hsu TC (2014) Efficiency improvement of a vertical light-emitting diode through surface plasmon coupling and grating scattering. Opt Express 22(S3):A842–A856
Lin CH, Su CY, Kuo Y, Chen CH, Yao YF, Shih PY, Chen HS, Hsieh C, Kiang YW, Yang CC (2014) Further reduction of efficiency droop effect by adding a lower-index dielectric interlayer in a surface plasmon coupled blue light-emitting diode with surface metal nanoparticles. Appl Phys Lett 105(10):101106
Yeh DM, Huang CF, Chen CY, Lu YC, Yang CC (2008) Localized surface plasmon-induced emission enhancement of a green light-emitting diode. Nanotechnology 19(34):345201
Kuo Y, Chen HT, Chang WY, Chen HS, Yang CC, Kiang YW (2014) Enhancements of the emission and light extraction of a radiating dipole coupled with localized surface plasmon induced on a surface metal nanoparticle in a light-emitting device. Opt Express 22(S1):A155–A166
Sun G, Khurgin JB, Yang CC (2009) Impact of high-order surface plasmon modes of metal nanoparticles on enhancement of optical emission. Appl Phys Lett 95(17):171103
Lu YC, Chen YS, Tsai FJ, Wang JY, Lin CH, Chen CY, Kiang YW, Yang CC (2009) Improving emission enhancement in surface plasmon coupling with an InGaN/GaN quantum well by inserting a dielectric layer of low refractive index between metal and semiconductor. Appl Phys Lett 94(23):233113
Chen CY, Wang JY, Tsai FJ, Lu YC, Kiang YW, Yang CC (2009) Fabrication of sphere-like Au nanoparticles on substrate with laser irradiation and their polarized localized surface plasmon behaviors. Opt Express 17(16):14186–14198
Zhang S, Watson S, McKendry JJD, Massoubre D, Cogman A, Gu E, Henderson RK, Kelly AE, Dawson MD (2013) 1.5 Gbit/s multi-channel visible light communications using CMOS-controlled GaN-based LEDs. J Lightwave Technol 31(8):1211–1216
Tian P, McKendry JJD, Gong Z, Zhang S, Watson S, Zhu D, Watson IM, Gu E, Kelly AE, Humphreys CJ, Dawson MD (2014) Characteristics and applications of micro-pixelated GaN-based light emitting diodes on Si substrates. J Appl Phys 115(3):033112
Liao CL, Chang YF, Ho CL, Wu MC (2013) High-speed GaN-based blue light-emitting diodes with gallium-doped ZnO current spreading layer. IEEE Electron Dev Lett 34(2):611–613
Zhu S, Wang J, Yan J, Zhang Y, Pei Y, Si Z, Yang H, Zhao L, Liu Z, Li J (2014) Influence of AlGaN electron blocking layer on modulation bandwidth of GaN-based light emitting diodes. ECS Solid State Lett 3(3):R11–R13
Huang CW, Tseng HY, Chen CY, Liao CH, Hsieh C, Chen KY, Lin HY, Chen HS, Jung YL, Kiang YW, Yang CC (2011) Fabrication of surface metal nanoparticles and their induced surface plasmon coupling with subsurface InGaN/GaN wells. Nanotechnology 22(47):475201
Chen HS, Yao YF, Liao CH, Tu CG, Su CY, Chang WM, Kiang YW, Yang CC (2013) Light-emitting device with regularly patterned growth of an InGaN/GaN quantum-well nanorod light-emitting diode array. Opt Lett 38(17):3370–3373
Khurgin JB, Sun G, Soref RA (2007) Enhancement of luminescence efficiency using surface plasmon polaritons: figures of merit. J Opt Soc Am B 24(8):1968–1980
Acknowledgments
This research was supported by Ministry of Science and Technology, Taiwan, The Republic of China, under the grants of NSC 102-2221-E-002-204-MY3, 102-2120-M-002-006, and 102-2221-E-002-199, by the Excellent Research Projects of National Taiwan University (103R890951 and 103R890952), and by US Air Force Scientific Research Office under the contract of AOARD-13-4143.
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
About this article
Cite this article
Lin, CH., Chen, CH., Yao, YF. et al. Behaviors of Surface Plasmon Coupled Light-Emitting Diodes Induced by Surface Ag Nanoparticles on Dielectric Interlayers. Plasmonics 10, 1029–1040 (2015). https://doi.org/10.1007/s11468-015-9902-9
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s11468-015-9902-9