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A Computational Approach Based on GIS Technology for the Development of an Anthropogenic Emission Inventory of Gaseous Pollutants in Greece

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Abstract

This paper describes a computational system developed for the compilation of an anthropogenic emission inventory of gaseous pollutants for Greece. The inventory was developed using a geographical information system integrated with SQL programming language to provide high temporal gridded emission fields for CO, NO2, NO, SO2, NH3 and 23 non-methane volatile organic compounds (NMVOCs) species for the reference year 2003. Activity and statistical data from national sources were used for the quantification of emissions from the road transport, the other mobile sources and machinery sectors and from range activities using top-down or bottom-up methodologies. Annual emission data from existing national and European emission databases were also used. The emission data were spatially and temporally disaggregated using source-specific spatiotemporal indicators. On national scale, the road transport sector produces about 60% of the annual CO and NMVOC total emissions, with gasoline vehicles being the main CO and NMVOC emissions source. The road transport is responsible for approximately half of the higher alkanes and for more than half of the ethene and toluene emissions. The maritime sector accounts for about 40% of the annual total NOx emissions, most of which are emitted by the international shipping subsector, whilst SO2 is emitted mainly by the energy sector. The evaluation of the emissions inventory suggests that it provides a good representation of the amounts of gaseous pollutants emitted on national scale and a good characterisation of the relative composition of CO and NOx emission in the large urban centres.

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References

  • Aleksandropoulou, V., & Lazaridis, M. (2004). Spatial distribution of gaseous and particulate matter emissions in Greece. Water, Air and Soil Pollution, 153, 15–34.

    Article  CAS  Google Scholar 

  • Borge, R., Lumbreras, J., & Rodriguez, E. (2007). Development of a high-resolution emission inventory for Spain using the SMOKE modelling system: A case study for the years 2000 and 2010. Environmental Modelling and Software, 23, 1026–1044.

    Google Scholar 

  • Brodie, R. S. (1999). Integrating GIS and RDBMS technology during construction of a regional groundwater model. Environmental Modelling and Software, 14, 119–128.

    Article  Google Scholar 

  • Brohan, P., Kennedy, J. J., Haris, I., Tett, S. F. B., & Jones, P. D. (2006). Uncertainty estimates in regional and global observed temperature changes: a new dataset from 1850. Journal of Geophysical Research, 111, D12106, doi:10.1029/2005JD006548.

  • Dai, J., & Rocke, D. M. (2000). A GIS-based approach to spatial allocation of area source solvent emissions. Environmental Modelling and Software, 15, 293–302.

    Article  Google Scholar 

  • EC (European Commission). (2000). Commission Decision 2000/479/EC of 17 July 2000 on the implementation of a European pollutant emission register (EPER) according to Article 15 of Council Directive 96/61/EC concerning integrated pollution prevention and control (IPPC). Official Journal of the European Communities L 192, pp. 36–43. http://eper.eea.europa.eu/eper/.

  • Economopoulou, A., & Economopoulos, A. (2002). Air pollution in Athens basin and health risks assessment. Environmental Monitoring and Assessment, 80, 277–299.

    Article  CAS  Google Scholar 

  • EEA (European Environment Agency). (2000). CORINE land cover technical guide—Addendum 2000. The European Topic Centre on Terrestrial Environment. EEA Technical Report no. 40.

  • EMEP/CORINAIR. (2001). Atmospheric emission inventory guidebook (3rd ed.). Copenhagen: European Environmental Agency.

    Google Scholar 

  • ENVIRON. (2004). Evaluation of the US EPA MOBILE6 highway vehicle emission factor model. Final report CRC project E64. http://www.epa.gov/otaq/models/mobile6/crce64.pdf.

  • Friedrich, R. (1997). GENEMIS: Assessment, improvement, temporal and spatial disaggregation of European emission data. In A. Ebel, R. Friedrich & H. Rhode (Eds.), Tropospheric modelling and emission estimation, (PART 2). New York: Springer.

    Google Scholar 

  • Funk, T. H., Chinkin, L. R., Roberts, P. T., Saeger, M., Mulligan, S., Paramo Figueroa, V. H., et al. (2001). Compilation and evaluation of a Paso del Norte emission inventory. Science of the Total Environment, 276, 135–151.

    Article  CAS  Google Scholar 

  • Ganev, K., Dimitrova, R., Syrakov, D., & Zerefos, C. (2003). Accounting for the mesoscale effects on the air pollution in some cases of large sulfur pollution in Bulgaria or Northern Greece. Environmental Fluid Mechanics, 3, 41–53.

    Article  CAS  Google Scholar 

  • Ganev, K., Prodanova, M., Syrakov, D., & Miloshev, N. (2008). Air pollution transport in the Balkan region and country-to-country pollution exchange between Romania, Bulgaria and Greece. Ecological Modelling, 217, 255–269.

    Article  CAS  Google Scholar 

  • Giannouli, M., Samaras, Z., Keller, M., deHaan, P., Kallivoda, M., Sorenson, S., et al. (2006). Development of a database system for the calculation of indicators of environmental pressure caused by transport. Science of the Total Environment, 357, 247–270.

    Article  CAS  Google Scholar 

  • Graedel, T. E., Bouwman, A. F., Gunnold, D., Dignon, J., Fung, I., Jacob, D. J., et al. (1993). A compilation of inventories of emissions to the atmosphere. Global Biogeochemical Cycles, 7, 1–26.

    Article  CAS  Google Scholar 

  • GSNSSG. (2003). General secretariat of the national statistical agency of Greece. http://www.statistics.gr/.

  • Hanna, S. R., Lu, Z., Frey, H. C., Wheeler, N., Vukovich, J., Arunachalam, S., et al. (2001). Uncertainties in predicted ozone concentrations due to input uncertainties for the UAM-V photochemical grid model applied to the July 1995 OTAG domain. Atmospheric Environment, 35, 891–903.

    Article  CAS  Google Scholar 

  • H.M.E.P.P.P.W. (2001). An inventory of the air pollutants and liquid and solid waste emitted from industry. An emission inventory of the central heating. Report of the Hellenic Ministry for the Environment, Physical Planning and Public Works, Report No YP4-PETREFREP-AWS-01-01.

  • HNSM (Hellenic National Meteorological Service). (2007). http://www.hnms.gr/hnms/english/climatology/climatology_html.

  • Houyoux, M. R., Vukovich, J. M., Coats, C. J., Jr., Wheeler, N. J. M., & Kasibhatla, P. S. (2000). Emission inventory development and processing for the Seasonal Model for Regional Air Quality (SMRAQ) project. Journal of Geophysical Research (D Atmosphere), 105, 9079–9090.

    Article  CAS  Google Scholar 

  • Katsoulis, D. B., & Whelpdale, D. M. (1990). Atmospheric sulphur and nitrogen budgets for Southeast Europe. Atmospheric Environment, 24A, 2959–2970.

    CAS  Google Scholar 

  • Kyriakis, N., Samaras, Z., Andrias, A. (1998). MEET: Road traffic composition. MEET deliverable 16. LAT report, n89823, Thessaloniki, Greece.

  • Lalas, D. P. (2001). Climate change, emission inventory, national inventory for greenhouse and other gases for the years 1990–1999. Technical Report of the National Observatory of Athens.

  • Mannschreck, K., Klemp, D., Kley, D., Friedrich, R., Kühlwein, J., Wickert, B., et al. (2002). Evaluation of an emission inventory by comparisons of modelled and measured emission ratios of individual HCs, CO and NOx. Atmospheric Environment, 36, 81–94.

    Article  Google Scholar 

  • Matzarakis, A., & Balafoutis, C. (2004). Heating degree days over Greece as an index of energy consumption. International Journal of Climatology, 24, 1817–1828.

    Article  Google Scholar 

  • Olivier, J. G. J., Berdowski, J. J. M., Peters, J. A. H. W., Bakker, J., Visschedijk, A. J. H., & Bloos, J.-P. J. (2001). Applications of EDGAR. Including a description of EDGAR 3.0: reference database with trend data for 1970–1995. RIVM, Bilthoven. RIVM report no. 773301 001/NOP report no. 410200 051.

  • Passant, N. R. (2003). Estimation of uncertainties in the National Atmospheric Emissions Inventory. AEAT/ENV/R/1039t.

  • Pham, T. B. T., Manomaiphiboon, K., & Vongmahadlek, C. (2008). Development of an inventory and temporal allocation profiles of emissions from power plants and industrial facilities in Thailand. Science of theTotal Environment, 397, 1–3.

    Article  CAS  Google Scholar 

  • Poupkou, A., Symeonidis, P., Ziomas, I., Melas, D., & Markakis, K. (2007). A spatially and temporally disaggregated anthropogenic emission inventory in the Southern Balkan region. Water, Air and Soil Pollution, 185, 355–348.

    Article  CAS  Google Scholar 

  • Poupkou, A., Melas, D., Ziomas, I., Symeonidis, P., Lisaridis, I., Gerasopoulos, E., et al. (2008). Simulated summertime regional ground-level ozone concentrations over Greece. Water, Air and Soil Pollution. doi:10.1007/s11270-008-9766-0.

    Google Scholar 

  • Poupkou, A., Symeonidis, P., Lisaridis, I., Melas, D., Ziomas, I., Yay, O. D., et al. (2008). Effects of anthropogenic emission sources on maximum ozone concentrations over Greece. Atmospheric Research, 89, 374–381.

    Article  CAS  Google Scholar 

  • Russell, A., & Dennis, R. (2000). NARSTO critical review of photochemical models and modelling. Atmospheric Environment, 34, 2261–2282.

    Article  Google Scholar 

  • Samaras, Z., Kyriakis, N., & Zachariadis, T. (1995). Reconciliation of macroscale and microscale motor vehicle emission estimates. Science of the Total Environment, 169, 231–239.

    Article  CAS  Google Scholar 

  • Schneider, C., Kessler, C., & Moussiopoulos, N. (1997). Influence of emission input data on ozone level predictions for the upper Rhine Valley. Atmospheric Environment, 31, 3187–3205.

    Article  CAS  Google Scholar 

  • Sotiropoulou, R. E. P., Tagaris, E., & Pilinis, C. (2004). An estimation of the spatial distribution of agricultural ammonia emissions in the Greater Athens Area. Science of the Total Environment, 318, 159–169.

    Article  CAS  Google Scholar 

  • Symeonidis, P. (2002). Study of the atmospheric pollution and its sources with the use of a geographical information system. Dissertation, Aristotle University of Thessaloniki.

  • Symeonidis, P., Ziomas, I., & Proyou, A. (2003). Emissions of air pollutants from the road transport sector in Greece: Year to year variation and present situation. Environmental Technology, 24, 719–725.

    Article  CAS  Google Scholar 

  • Symeonidis, P., Ziomas, I., & Proyou, A. (2004). Development of an emission inventory system for transport in Greece. Environmental Modelling and Software, 9, 413–421.

    Google Scholar 

  • Symeonidis, P., Poupkou, A., Gkantou, A., Melas, D., Yay, O. D., Pouspourika, Ε., et al. (2008). Development of a computational system for estimating biogenic NMVOCs emissions based on GIS technology. Atmospheric Environment, 42, 1777–1789.

    Article  CAS  Google Scholar 

  • Taghavi, M., Cautenet, S., & Arteta, J. (2005). Impact of highly detailed emission inventory on modelling accuracy. Atmospheric Research, 74, 65–68.

    Article  CAS  Google Scholar 

  • Tsilingiridis, G., Zachariadis, T., & Samaras, Z. (2002). Spatial and temporal characteristics of air pollutant emissions in Thessaloniki, Greece: Investigation of emission abatement measures. Science of the Total Environment, 300, 99–113.

    Article  CAS  Google Scholar 

  • USEPA. (1996). PAMS 1996 Data analysis report. Report EPA 454/R-96-006, Chapter 3, p. 44, Office of Air Quality Planning and Standards, Research Triangle Park, NC. http://pubweb.epa.gov/air/oaqps/pams/pamsrr.html.

  • USEPA. (2002). SPECIATE database V3.2. http://www.epa.gov/ttn/chief/software/speciate.

  • USEPA. (2004). Median life, annual activity, and load factor values for non-road engine emissions modeling. NR-005c (EPA420-P-04-005, April 2004). http://www.epa.gov/otaq/models/nonrdmdl/nonrdmdl2004/420p04005.pdf.

  • Vestreng, V., Rigler, E., Adams, M., Kindbom, K., Pacyna, J.M., van der Gon, H.D.r, Reis, S., Travnikov, O. (2006). Inventory review 2006. Emission data reported to LRTAP Convention and NEC Directive. Initial review of HMs and POPs. Technical report MSC-W 1/2006.

  • Visschedijk, A. J. H., Zandveld, P. Y. J., & Denier van der Gon, H. A. C. A. (2007). High resolution gridded European emission database for the EU integrate project GEMS. TNO-report 2007-A-R0233/B.

  • Zanis, P., Katragkou, E., Kanakidou, M., Psiloglou, B. E., Karathanasis, S., Vrekoussis, M., et al. (2007). Effects on surface atmospheric photo-oxidants over Greece during the total solar eclipse event of 29 March 2006. Atmospheric Chemistry and Physics, 7, 6061–6073.

    Article  CAS  Google Scholar 

  • Ziomas, I., Suppan, P., Rappengluck, B., Balis, D., Tzoumaka, P., & Melas, D. (1995). A contribution to the study of photochemical smog in the Greater Athens Area. Beitraege zur Physiologie Atmosphere, 68, 191–203.

    Google Scholar 

  • Ziomas, I., Tzoumaka, P., Balis, D., Melas, D., Zerefos, C., & Klemm, O. (1998). Ozone episodes in Athens, Greece. A modelling approach using data from the MEDCAPHOT-TRACE. Atmospheric Environment, 32, 2313–2321.

    Article  CAS  Google Scholar 

  • Zoras, S., Triantafyllou, A. G., & Evagelopoulos, V. (2006). Modelling of PM2.5 episodes in four cities of northwestern Greece. Fresenius Environmental Bulletin, 15, 306–313.

    CAS  Google Scholar 

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Acknowledgements

The research study was financed by the Greek Ministry of Education (research project PROMOTE II).

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Correspondence to Konstantinos Markakis.

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Markakis, K., Poupkou, A., Melas, D. et al. A Computational Approach Based on GIS Technology for the Development of an Anthropogenic Emission Inventory of Gaseous Pollutants in Greece. Water Air Soil Pollut 207, 157–180 (2010). https://doi.org/10.1007/s11270-009-0126-5

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