Skip to main content

Advertisement

Log in

Accelerated methane oxidation cover system to reduce greenhouse gas emissions from MSW landfills in cold, semi-arid regions

  • Published:
Water, Air, and Soil Pollution Aims and scope Submit manuscript

Abstract

Many regional landfills for municipal solid waste (MSW) and industrial, commercial, institutional (ICI) wastes in cold, dry regions do not produce enough gas to support conventional gas extraction, treatment, and utilization or flaring. Yet, some solution is required to reduce emissions of methane and trace constituents to the atmosphere for the protection of the public and of the global climate. Methane oxidation, as a natural biochemical process, offers an opportunity to reduce methane emissions with a simple, passive alternative cover system. The goal of this article is to develop an effective design of Methane Oxidation Covers to achieve superior methane management performance while still producing equivalent closure conditions to conventional covers in semi-arid, cold climates. specifically, the goal is to reduce methane surface emissions by 50% to 80%, with no significant increase in leachate production compared with conventional covers of clay and topsoil.

A field pilot test of an alternative cover system with gas collection, methane oxidation and heat extraction was conducted on an operating MSW/ICI waste landfill in Western Canada from August 2001 to February 2005. The cool, semi-arid region experiences cold winters (down to minus 40˚C) for up to 5 months of the year, and annual precipitation rates of 150 mm to 450 mm p.a., of which one third to one half falls as snow.

The need to direct gas from large surface areas to gas control zones of minimal area led to the configuration of the system of gas collection trenches connected to a central methane oxidation (MethOx) bed. The need to keep the bed above 5˚C in winter required the development of a simple, passive heat transfer system.

The maintenance of suitable moisture contents and the restriction of percolation were accomplished by the choice of filter material and the layering of the bed over the gas percolation layer.

The test program was conducted in three phases from August 2001 to February 2005. In the first test phase, a methane oxidation bed of yardwaste compost performed well during the summer, but froze from November to April and did not resume oxidation until May. Oxygen was always present at or above 3%(vol.) and the moisture content remained above 25%(vol.) in the lower layer of the bed. The freezing temperature caused the most serious performance reduction. In the next phases of the study, a passive heating system was installed in an accelerated methane oxidation bed. Heat exchange from inside the landfill to the filter raised the bed temperature to 14 to 18˚C during the third winter of the test. The moisture contents of 25% to 50% (v/v) in the bed were high, but the percolation rate was only 7.3 mm/a, or about 2% of total precipitation. The methane oxidation performance increased with the heating of the bed, from a 33% emission reduction in an unheated bed, up to 89% in a well heated filter bed. The achievement of high oxidation performance (over 80%), the complete reduction of surface emissions from the test area (to zero), and the low percolation rate through the filter bed (less that 2%) constitute a proof of principle for MethOx covers in cool, semi-arid climates. The possible improvement of the Alternative Cover System's performance by adding vegetation to the filter bed is currently being tested in the ongoing research project.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  • Albright, W., Benson, C., Gee, G., Roesler, A., Abichou, T., Apiwantragoon, P., Lyles, B., & Rock, S. (2004). Field water balance of landfill final covers. J. Environ. Qual., 33, 2317–2332.

    PubMed  CAS  Google Scholar 

  • Boeckx, P., & van Cleemput, O. (1996). Methane oxidaiton in a landfill cover soil: influence of moisture content, temperature, and nitrogen turnover. J. Environ. Qual., 25, 178–183.

    CAS  Google Scholar 

  • Borjesson, G., Sundh, I., & Svensson, B. (2004). Microbial oxidation of CH4 at different temperatures in landfill cover soils. FEMS Microbiol. Ecol., 48, 305–312.

    Article  CAS  PubMed  Google Scholar 

  • Borjesson, G., Danielsson, A., & Svensson, B. (2000). Methane fluxes from a swedish landfill by geostatistical treatment of static chamber measurements. Envir. Sci. Technol., 34, 4044–4050.

    Article  CAS  Google Scholar 

  • Borjesson, G., & Svensson, B. (1997). Seasonal and diurnal methane emissions from a landfill and their regulation by methane oxidation. Waste Management Res., 15, 33–54.

    Article  Google Scholar 

  • Christophersen, M., Linderoed, L., Jensen, P., & Kjeldsen, P. (2004). Methane oxidation at low temperatures in soil exposed to landfill gas. J. Environ. Qual., 29, 1989–1997.

    Article  Google Scholar 

  • Czepiel, P., Mosher, B., Crill, P., & Harriss, R. (1996). Quantifying the effect of oxidation on landfill methane emissions. J. Geophys. Res. Atmos., 101, 16721–16729.

    Article  CAS  ADS  Google Scholar 

  • DeVisscher, A., Thomas, D., Boecckx, P., & van Cleemput, O. (1999). Methane oxidation in simulated landfill cover soil environments, Environ. Sci. Technol., 33, 1854–1859.

    Article  CAS  Google Scholar 

  • Humer, M., & Lechner, P. (1999). Methane oxidation in compost cover layers on landfills, Proc. sardinia 99, 7 th Intl. waste management and landfill symposium, Cagliari, IT, Oct. 1999, 10 pp.

  • Nesbit, S. (1992). A laboratory study of factors influencing methane uptake by soils. Agriculture, Ecosystem and Environment, 41, 39–54.

    Article  CAS  Google Scholar 

  • Nozhevnikova, A., Lifshitz, A., Lebedev, V., & Zavarzin, G. (1993). Emission of methane into the atmosphere from landfills in the former USSR, Chemosphere, 26, 1–4, 401–417.

  • Omelchenko, M., Saleva, N., Vasilev, L., & Zavarkin, G. (1992). A psychrophilic methanotrophic community from tundra soil. Mikrobiologiya (Engl. Transl.), 61, 755–759.

    Google Scholar 

  • Oxford Canadian Atlas (2003). Toronto, Ont.: Oxford Univ. Press.

  • Park, S.-Y., Brown, K., & Thomas, J. (2004). The use of biofilters to reduce atmospheric methane emissions from landfills: Part 1 biofilter design. Water, Air and Soil Pollution, 155, 63–85.

    Article  CAS  Google Scholar 

  • Park, J.-W., & Shin, H.-C. (2001). Surface emission of landfill gas from solid waste landfills. Atmosph. Environment, 35, 3445–3451.

    Article  CAS  Google Scholar 

  • Scheutz, C., Moesbroek, H., & Kjeldsen, P. (2004). Attenuation of methane and volatile compounds in landfill cover soils. J. Environ. Qual., 33, 61–71.

    PubMed  CAS  Google Scholar 

  • Scheutz, C., Moesbroek, H., & Kjeldsen, P. (2004). Environmental factors influencing the attenuation of methane and hydrofluorocarbons in landfill cover soils. J. Environ. Qual., 33, 72–79.

    Article  PubMed  CAS  Google Scholar 

  • Schroeder, P., Dozier, T., Zappi, P., McEnroe, B., Sjostrom, J., Peyton, R. L. (1994). HELP model engineering documentation for Version 3. USEPA office of research and development, Cincinnati, OH, EPA/600/R-94/168b.

  • Sitaula, B., Bakken, L., & Abrahamsen, G. (1995). CH 4 uptake by temperate forest soil: effect of N input and soil acidification. Soil. Biol. Biochem., 27(7), 871–880.

    Article  CAS  Google Scholar 

  • Vecherskaya, M., Galchenko, V., Sokolova, E., & Samarkin, V. (1993). Activity and species composition of aerobic methanotrophic communities in tundra soil. Curr. Microbiol., 27, 181–187.

    Article  CAS  Google Scholar 

  • Whalen, S., Reeburgh, W., & Sandbeck, K. (1990). Rapid methane consumption in a landfill cover soil. Appl. Environ. Microbiol., 56, 3405–3411.

    PubMed  CAS  Google Scholar 

  • Zeiss, C. (2005). Accelerated methane oxidation in landfill covers in cold and dry regions, proc. 20 th intl. conf. on solid waste technology and management, Phila., Penn., April 3–6, 2005, 10 pp.

  • Zeiss, C., & Bajic, Z. (2001), Methane oxidation covers as an engineered greenhouse gas reduction measure for MSW landfills. Research Report CRD Research Project, University of Alberta, Jan. 31, 2001, 52 pp.

  • Zeiss, C., & Bajic, Z. (2000). Initial Greenhouse Gas Emission Assessment for A Regional Landfill in Western Canada. FCM GMEF Fund, Ottawa, Ont., July 2000, 39 pp.

  • Zeiss, C., & Bajic, Z. (1999). Landfill gas extraction as a greenhouse gas reduction method, in proc. 15 th intl. conference on solid waste technology and management, Widener Univ., Phildephia, Penn., Dec. 12–15, 1999, 10 pp.

    Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Rights and permissions

Reprints and permissions

About this article

Cite this article

Zeiss, C.A. Accelerated methane oxidation cover system to reduce greenhouse gas emissions from MSW landfills in cold, semi-arid regions. Water Air Soil Pollut 176, 285–306 (2006). https://doi.org/10.1007/s11270-006-9169-z

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s11270-006-9169-z

Keywords

Navigation