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Phase transition, microstructure and microwave dielectric properties of α-CaSiO3 ceramics with SiO2 addition

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Abstract

The effect of SiO2 addition on phase transition, microstructure and microwave dielectric properties of α-CaSiO3 ceramics was reported for the first time. The X-ray diffraction analysis confirmed that the phase transformation from cyclo-CaSiO3 to pseudo-CaSiO3 was inhibited with the increase of SiO2 content. It was observed that the average grain size decreased with the increasing addition of SiO2 by scanning electron microscope. The τ f of the SiO2-added α-CaSiO3 ceramics almost remained constant with the SiO2 content increased, while the ε r and Q × f changed obviously. The optimized properties were determined for SiO2 6 wt% additive α-CaSiO3 ceramics sintered at 1,350 °C: ε r  = 7.37, Q × f = 33,714 GHz and τ f  = −11.08 ppm/°C.

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References

  1. X.M. Xue, H.T. Yu, G.L. Xu, J. Mater. Sci. Mater. Electron. 24, 1287 (2013)

    Article  Google Scholar 

  2. P.S. Anjana, T. Joseph, M.T. Sebastian, Ceram. Int. 36, 1535 (2010)

    Article  Google Scholar 

  3. J. Liang, W.Z. Lu, W. Lei, G.F. Fan, H.R. Ma, J. Mater. Sci. Mater. Electron. 24, 3625 (2013)

    Article  Google Scholar 

  4. M. Li, W.Z. Lu, W. Lei, X.H. Wang, J.M. Wu, J. Mater. Sci. Mater. Electron. 24, 2672 (2013)

    Article  Google Scholar 

  5. H.P. Wang, J.M. Chen, W.Y. Yang, S.Q. Feng, H.P. Ma, G.H. Jia, S.Q. Xu, J. Eur. Ceram. Soc. 32, 541 (2012)

    Article  Google Scholar 

  6. Q.H. Yang, H.P. Wang, Z.P. He, D.H. Li, Q.H. Wang, S.Q. Xu, J. Ceram. Soc. Jpn. 122, 125 (2014)

    Article  Google Scholar 

  7. L. Jiao, S.P. Wu, X.H. Ding, J. Ni, J. Mater. Sci.: Mater. Electron. 20, 1186 (2009)

    Google Scholar 

  8. N. Mori, Y. Sugimoto, J. Harada, Y. Higuchi, J. Eur. Ceram. Soc. 26, 1925 (2006)

    Article  Google Scholar 

  9. J.Y. Wu, J.J. Bian, Ceram. Int. 38, 3217 (2012)

    Article  Google Scholar 

  10. K.X. Song, X.M. Chen, X.C. Fan, J. Am. Ceram. Soc. 90, 1808 (2007)

    Article  Google Scholar 

  11. N. Tangboriboon, T. Khongnakhon, S. Kittikul, R. Kunanuruksapong, A. Sirivat, J. Sol-Gel Sci. Technol. 58, 33 (2011)

    Article  Google Scholar 

  12. P.N. De Aza, Z.B. Luklinsk, M.R. Anseau, M. Hector, F. Guitian, S. De Aza, Biomaterials 21, 1735 (2000)

    Article  Google Scholar 

  13. R.P.S. Chakradhar, B.M. Nagabhushana, G.T. Chandrappa, K.P. Ramesh, J.L. Rao, Mater. Chem. Phys. 95, 169 (2006)

    Article  Google Scholar 

  14. H.P. Sun, Q.L. Zhang, H. Yang, J.L. Zou, Mater. Sci. Eng. B 138, 46 (2007)

    Article  Google Scholar 

  15. H.P. Wang, Z.P. He, D.H. Li, R.S. Lei, J.M. Chen, S.Q. Xu, Ceram. Int. 40, 3895 (2014)

    Article  Google Scholar 

  16. W. Hu, H.X. Liu, H. Hao, Z.H. Yao, M.H. Cao, Z.J. Wang, Z. Song, J. Mater. Sci. Mater. Electron. 25, 4730 (2014)

    Article  Google Scholar 

  17. U.C. Chung, C. Elissalde, S. Mornet, M. Maglione, C. Estournes, Appl. Phys. Lett. 94, 072903 (2012)

    Article  Google Scholar 

  18. Z. Song, H.X. Liu, S.J. Zhang, Z.J. Wang, Y.T. Shi, H. Hao, M.H. Cao, Z.H. Yao, Z.Y. Yu, J. Eur. Ceram. Soc. 34, 1209 (2014)

    Article  Google Scholar 

  19. M.H. Frey, D.A. Payne, Phys. Rev. B 54, 3158 (1996)

    Article  Google Scholar 

Download references

Acknowledgments

This work was supported by the Key program of Natural Science Foundation of China (No. 50932004), International Science and Technology Cooperation Program of China (2011DFA52680), Natural Science Foundation of China (No. 51102189, No. 51372191), National Key Basic Research Program of China (No. 2015CB654601) and the program for New Century Excellent Talents in University (No. NCET-11-0685).

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Authors and Affiliations

  1. State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan, 430070, Hubei, People’s Republic of China

    Wei Hu, Hanxing Liu, Hua Hao, Zhonghua Yao, Minghe Cao, Zhijian Wang, Zhe Song & Haobo He

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  1. Wei Hu
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  2. Hanxing Liu
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  3. Hua Hao
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  4. Zhonghua Yao
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  5. Minghe Cao
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  7. Zhe Song
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  8. Haobo He
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Correspondence to Hanxing Liu.

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Hu, W., Liu, H., Hao, H. et al. Phase transition, microstructure and microwave dielectric properties of α-CaSiO3 ceramics with SiO2 addition. J Mater Sci: Mater Electron 26, 1977–1981 (2015). https://doi.org/10.1007/s10854-014-2637-0

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  • DOI: https://doi.org/10.1007/s10854-014-2637-0

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