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Characterization of radionuclide activity concentrations and lifetime cancer risk due to particulate matter in the Singrauli Coalfield, India

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Abstract

In this study, the activities of 40K, 210Pb, 232Th, 234U, 235U, and 238U in size-segregated particulate matter (PM) were measured in the Singrauli Coalfield, India. Different isotopic compositions were found relative to natural uranium ratios. The radioactivity concentration ratios in different PM sizes [PM2.5, PM10, and suspended particulate matter (SPM)] suggested that anthropogenic sources affected the uranium isotopic compositions in the area. A different isotopic composition from the natural uranium composition was found. The correlation coefficients between the measured isotopes (40K, 210Pb, 232Th, 234U, 235U, and 238U) and meteorological factors were calculated. PM emissions were affected by the meteorological conditions, which in turn, influenced the U and Th concentrations in PM. The 232Th/238U activity ratio in particulate matter was between 0.20 and 1.54 with an average value of 0.9 ± 0.5, 0.2 to 1.1 (0.8 ± 0.7), and 0.2 to 1.2 with an average value of 0.8 ± 0.8 in PM2.5, PM10, and SPM, respectively. These range were quite different from the average crustal ratio of 3.5, indicating that the 238U concentrations were elevated in this region relative to Th. However, compared with Th, the dose contribution of U to the public was negligible. The average effective dose in public owing to inhalation of natural radioactive 40K, 210Pb, 232Th, and 234U, 235U, and 238U in the atmosphere was between 0.03 and 327 nSv year−1. These doses associated with the inhalation of particulate matter were lower than world airborne reference value as reported by UNSCEAR (2000a).

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Acknowledgments

The corresponding author would like to express the highest gratitude to Indian Institute of Technology (Banaras Hindu University) and other organizations that helped me in this research work such as Northern Coalfield Limited, Singrauli; National Thermal Power Corporation Limited, Shaktinagar, Sonebhadra; Ministry of Human Resource Development, Government of India; and Bhabha Atomic Research Centre, Mumbai, Government of India.

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Authors and Affiliations

  1. Department of Mining Engineering, Indian Institute of Technology (Banaras Hindu University), Varanasi, 221 005, India

    Akhilesh Kumar Yadav

  2. Department of Public Health Sciences, University of Rochester School of Medicine and Dentistry, Rochester, NY, 14642, USA

    Philip Karl Hopke

  3. Institue for a Sustainable Environment, Clarkson University, Potsdam, NY, 13699, USA

    Philip Karl Hopke

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  1. Akhilesh Kumar Yadav
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Correspondence to Akhilesh Kumar Yadav.

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Highlights

• Radioactivity concentration in particulate matters increased as November to May.

• Radioactivity concentration influenced by particulate matters and meteorological factors.

• Mean 40K, 210Pb, 232Th, 234,235,238U were below global average values.

• The estimated lifetime cancer risk is 2.9 × 10−04 exceeded typical PM2.5 and PM10.

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Yadav, A.K., Hopke, P.K. Characterization of radionuclide activity concentrations and lifetime cancer risk due to particulate matter in the Singrauli Coalfield, India. Environ Monit Assess 192, 680 (2020). https://doi.org/10.1007/s10661-020-08619-1

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