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Effects of Synthesis Routes on the States and Catalytic Performance of Manganese Oxides Used for Diesel Soot Combustion

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Abstract

The catalyst obtained through the co-precipitation of Mn(Ac)2 and (NH4)2CO3 (denoted as Mn–Ac–NH4) displays the highest performance for soot oxidation. Compared with other MnOx catalysts, the catalyst Mn–Ac–NH4 exhibits much better reducibility and more uniform sponge-like nanostructure. The characterization results indicate that the oxygen species on the surface of Mn–Ac–NH4 are more active for soot combustion. The NO species can also be captured and oxidized by these oxygen species, generating more reactive NO2 which can enhance soot oxidation.

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Acknowledgments

This work is financially supported by the National Natural Science Foundation of China (21276184, U1332102), the Specialized Research Fund for the Doctoral Program of Higher Education of China (20120032110014) and the Program of Introducing Talents of Discipline to University of China (No. B06006).

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Authors and Affiliations

  1. Collaborative Innovation Center for Chemical Science and Engineering (Tianjin), Tianjin Key Laboratory of Applied Catalysis Science and Engineering, School of Chemical Engineering and Technology, Tianjin University, Tianjin, 300072, People’s Republic of China

    Fangfang Dai, Yifu Yu & Ming Meng

  2. Institute of High Energy Physics, Chinese Academy of Sciences, Beijing, 100049, People’s Republic of China

    Jing Zhang, Lirong Zheng & Tiandou Hu

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  1. Fangfang Dai
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  2. Yifu Yu
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  3. Ming Meng
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  4. Jing Zhang
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  5. Lirong Zheng
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  6. Tiandou Hu
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Correspondence to Ming Meng.

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Dai, F., Yu, Y., Meng, M. et al. Effects of Synthesis Routes on the States and Catalytic Performance of Manganese Oxides Used for Diesel Soot Combustion. Catal Lett 144, 1210–1218 (2014). https://doi.org/10.1007/s10562-014-1268-7

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  • DOI: https://doi.org/10.1007/s10562-014-1268-7

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