Skip to main content
Log in

Sinking of particulates 234Thxs, 7Be and 210Pbxs in the Changjiang estuary, China

  • Chemistry
  • Published:
Chinese Journal of Oceanology and Limnology Aims and scope Submit manuscript

Abstract

The time scale of transport and reaction processes in the ocean can be evaluated using natural radionuclides of different half-lives. In the present study, we evaluated the residence times of particulate reactive radionuclides 7Be, 210Pbxs and 234Th in the Changjiang (Yangtze River) estuary, which is a high turbidity estuary, in June, 2006. The residence times of particulate 7Be, 234Thxs and 210Pbxs in the Changjiang estuary were calculated to be 0.7–20.4, 0.18–4.1 and 0.6–89.8 d, respectively. The obtained residence times of those nuclides are comparable with those of other estuaries and bays. For 234Thxs and 7Be, the residence times decreased with increasing concentrations of suspended particulate matter (SPM); however, those of 210Pbxs increased. Moreover, scavenging residence times of 234Th and 7Be increased from coast to offshore, while those of 210Pbxs decreased.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  • Aller R C, Cochran J K. 1976. 234Th/238U disequilibrium in nearshore sediment: particle reworking and digenetic timescales. Earth and Planetary Science Letters, 29: 37–50.

    Article  Google Scholar 

  • Baskaran M, Santschi P H. 1993a. The role of particles and colloids in the transport of radionuclides in coastal environments of Texas. Marine Chemistry, 43: 95–114.

    Article  Google Scholar 

  • Baskaran M, Coleman C H, Santschi P H. 1993b, Atmospheric depositional fluxes of 7Be and 210Pb at Galveston and College Station, Texas. Journal of Geophysical Research, 98:20 555–20 571.

    Article  Google Scholar 

  • Baskaran M, Swarzenski P W. 2007. Seasonal variations on the residence times and partitioning of short-lived radionuclides (234Th, 7Be and 210Pb) and depositional fluxes of 7Be and 210Pb in Tampa Bay, Florida. Marine Chemistry, 104: 27–42.

    Article  Google Scholar 

  • Baskaran M, Santschi P H, Guo L, Bianchi T S, Lambert C. 1996. 234Th-238U disequilibria in the Gulf of Mexico: the importance of organic matter and particle concentration. Continental Shelf Research, 16: 353–380.

    Article  Google Scholar 

  • Baskaran M, Ravichandran M, Bianchi T S. 1997. Cycling of 7Be and 210Pb in a high DOC, shallow, turbid estuary of southeast Texas. Estuarine, Coastal and Shelf Science, 45: 165–176.

    Article  Google Scholar 

  • Bronson F L. 2003. Validation of the accuracy of the LabSOCS software for mathematical efficiency calibration of Ge detectors for typical laboratory samples. Journal of Radioanalytical and Nuclear Chemistry, 255(1): 137–141.

    Article  Google Scholar 

  • Chen M, Huang Y P, Qiu Y. 2001. Tidal effect on 234Th/238U disequilibria in Xiamen Bay. Oceanologia et Limnologia Sinica, 32(6): 679–689. (in Chinese)

    Google Scholar 

  • Dai Z, Du J, Li J, Li W, Chen J. 2008. Runoff characteristics of the Changjiang River during 2006: Effect of extreme drought and the impounding of the Three Gorges Dam. Geophysical Research Letters, 35: L07406, doi:10.1029/2008GL033456.

    Article  Google Scholar 

  • Dibb J E, Rice D L. 1989. The geochemistry of beryllium-7 in Chesapeake Bay. Estuarine and Coastal Shelf Science, 28: 379–394.

    Article  Google Scholar 

  • Du J, Zhang J, Zhang J, Wu Y. 2008. Deposition patterns of atmospheric 7Be and 210Pb in coast of East China Sea, Shanghai, China. Atmospheric Environment, 42: 5 101–5 109.

    Google Scholar 

  • Feng H, Cochran J K, Hirschberg D J, Wilson R E. 1998. Small-scale spatial variations of natural radionuclide and trace metal distributions in sediments from the Hudson River estuary. Estuaries, 21: 263–280.

    Article  Google Scholar 

  • Feng H, Cochran J K, Hirschberg D J. 1999. 234Th and 7Be as traces for the transport and dynamics of suspended particles in a partially mixed estuary. Geochimica et Cosmochimica Acta, 63: 2 487–2 505.

    Google Scholar 

  • Hirschberg D J, Chin P, Feng H, Cochran J K. 1996. Dynamics of sediment and contaminant transport in the Hudson River estuary. Evidence from sediment distribution of naturally occurring radionuclides. Estuaries, 19: 175–193.

    Article  Google Scholar 

  • Ivanovich M, Harmon R S. 1992. Uranium-series Disequilibrium: Application to Earth, Marine and Environmental Sciences, 2nd ed. Clarendon Press, Oxford, p. 731–778.

    Google Scholar 

  • Jweda J, Baskaran M, van Hees E, Schweitzer L. 2008. Short-lived radionuclides (Be-7 and Pb-210) as tracers of particle dynamics in a river system in southeast Michigan, Limnology and Oceanography, 53(5): 1 934–1 944.

    Google Scholar 

  • Kaufman A, Li Y H, Turekian K K. 1981. The removal rates of 234Th and 228Th from waters of the New York Bight. Earth and Planetary Science Letters, 54(3): 385–392.

    Article  Google Scholar 

  • Liu J, Li A, Xu K, Velozzi D M, Yang Z, Milliman J D, DeMaster D J. 2006. Sedimentary features of the Yangtze River-derived along-shelf clinoform deposit in the East China Sea. Continental Shelf Research, 26: 2 141–2 156

    Article  Google Scholar 

  • Liu J, Xu K, Li A, Milliman J D, Velozzi D M, Xiao S B, Yang Z S. 2007. Flux and fate of Yangtze River sediment delivered to the East China Sea. Geomorphology, 85: 208–224.

    Article  Google Scholar 

  • McKee B A, DeMaster D J, Nittrouer C A. 1984. The use of Th-234/U-238 disequilibrium to examine the fate of particle-reactive species in the Yangtze continental shelf. Earth and Planetary Science Letters, 68: 431–442.

    Article  Google Scholar 

  • McKee B A, DeMaster D J, Nittrouer C A. 1986. Temporal variability in the partitioning of thorium between dissolved and particulate phases of the Amazon shelf: implications for the scavenging of particle-reactive species. Continental Shelf Research, 6: 87–106.

    Article  Google Scholar 

  • Olsen C R, Larsen I L, Lowry P D, Cutshall N H, Nichols M M. 1986. Geochemistry and deposition of 7Be in river-estuarine and coastal waters. Journal Geophysical Research, 91(C1): 896–908.

    Article  Google Scholar 

  • Preiss N, Meliees M A, Pourchet M A. 1996. Compilation of data on lead-210 concentration in surface air and fluxes at the air-surface and water-sediment interfaces. Journal of Geophysical Research, 101: 28 847–28 862.

    Article  Google Scholar 

  • Santschi P H, Li Y H, Bell J. 1979. Natural radionuclides in the water of Narragansett Bay. Earth and Planetary Science Letters, 45: 201–213.

    Article  Google Scholar 

  • Shen H, Pan D. 2001. Turbidity Maximum in the Changjiang Estuary, China Ocean Press, Beijing, China. Chapter 3. (in Chinese)

    Google Scholar 

  • Tan X, Wang X, Gechies H, Rabung A. 2008. Sorption of Eu(III) on humic acid or fulvic acid bound to hydrous alumina studied by SEM-EDS, XPS, TRLFS, and batch techniques. Environmental Science & Technology, 42: 6 532–6 537.

    Google Scholar 

  • Turner A, Millward G E. 2002. Suspended particles: their role in estuarine biogeochemical cycles. Estuarine, Coastal and Shelf Science, 55: 165–176.

    Article  Google Scholar 

  • Wong C M, Williams C E, Pittock J, Collier U, Schelle P. 2007. World’s Top 10 Rivers at Risk. WWF International. Gland, Switzerland.

    Google Scholar 

  • Wu Y, Zhang J, Li D, Wei H, Lu R. 2003. Isotope variability of particulate organic matter at the PN Section in the East China Sea. Biogeochemistry, 65: 31–49.

    Article  Google Scholar 

  • Xu D, Chen C, Tan X, Hu J, Wang X. 2007. Sorption of Th(IV) on Na-rectorite: Effect of HA, ionic strength, foreign ions and temperature. Applied Geochemistry, 22: 2 892–2 906.

    Article  Google Scholar 

  • Yang S, Zhang J, Zhu J, Smith J P, Dai S, Gao A, Li P. 2005. Impact of dams on Yangtze River sediment supply to the sea and delta inter-tidal wetland response. Journal of Geophysical Research, 110: F03006, doi: 0.1029/2004JF000271.

    Article  Google Scholar 

  • Yang S, Zhang J, Xu X. 2007. Influence of the Three Gorges Dam on downstream delivery of sediment and its environmental implications, Yangtze River, Geophysical Research Letters, 34: L10401, doi:10.1029/2007GL029472.

    Article  Google Scholar 

  • Zhang J. 2002. Biogeochemistry of Chinese estuarine and coastal waters: Nutrients, trace metals and biomarkers. Regional Environmental Change, 3: 65–76.

    Article  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Jinzhou Du  (杜金洲).

Additional information

Supported by the National Natural Science Foundation of China (No. 40976054), the State Key Laboratory of Estuarine and Coastal Research of China (No. 2008KYYW08), and the National Basic Research Program of China (973 Program) (Nos. 2002CB412405 and 2006CB400601)

Rights and permissions

Reprints and permissions

About this article

Cite this article

Huang, D., Du, J., Wu, Y. et al. Sinking of particulates 234Thxs, 7Be and 210Pbxs in the Changjiang estuary, China. Chin. J. Ocean. Limnol. 28, 1152–1159 (2010). https://doi.org/10.1007/s00343-010-9036-z

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s00343-010-9036-z

Keyword

Navigation