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Dynamic response of converse magnetoelectric effect in a PMN-PT-based multiferroic heterostructure

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Abstract

A multiferroic heterostructure, consisting of a 25 μm thick Metglas® ribbon affixed to a lead magnesium niobate–lead titanate (PMN-PT) crystal, was systemically studied to investigate the time response of converse magnetoelectric coupling under the application of electric fields at low frequencies (0.05<f<10 Hz). This multiferroic heterostructure exhibits a considerably strong converse magnetoelectric effect, CME=−80%, where CME=[M(E)−M(0)]/M(0), and a converse ME coupling constant, A=22.5 Oe-cm/kV, at frequencies below 1 Hz and near saturation electric polarization. A switching time (t s), representing the response time of the CME coupling, is measured to be 0.6 seconds for this heterostructure under the application of instantaneous electric fields. The switching time results in significant influences on the magnetoelectric effect especially at frequencies higher than 2 Hz. The dynamic response of CME coupling is predominantly determined by ferroelectric relaxation within the PMN-PT crystal, as opposed to the magnetic relaxation of the Metglas® ribbon. A model was used to describe the dynamic behavior of CME coupling in disordered systems such as PMN-PT.

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References

  1. J. Scott, Nat. Mater. 6, 256 (2007)

    Article  ADS  Google Scholar 

  2. W. Eerenstein, M. Wiora, J.L. Prieto, J.F. Scott, N.D. Mathur, Nat. Mater. 6, 351 (2007)

    Article  ADS  Google Scholar 

  3. T. Kimura, Annu. Rev. Mater. Res. 37, 387 (2007)

    Article  ADS  Google Scholar 

  4. R. Ramesh, N.A. Spaldin, Nat. Mater. 6, 21 (2007)

    Article  ADS  Google Scholar 

  5. Y. Chen, J. Gao, T. Fitchorov, Z. Cai, K.S. Ziemer, C. Vittoria, V.G. Harris, Appl. Phys. Lett. 94, 082504 (2009)

    Article  ADS  Google Scholar 

  6. Y. Chen, J. Gao, J. Lou, S.D. Yoon, A.L. Geiler, M. Nedoroscik, D. Heiman, N.X. Sun, C. Vittoria, V.G. Harris, J. Appl. Phys. 105, 07A510 (2009)

    Article  Google Scholar 

  7. D.A. Filippov, G. Srinivasan, A. Gupta, J. Phys. Condens. Matter. 20, 425206 (2008)

    Article  ADS  Google Scholar 

  8. Y.K. Fetisov, G. Srinivasan, Appl. Phys. Lett. 88, 143503 (2006)

    Article  ADS  Google Scholar 

  9. A.S. Tatarenko, G. Srinivasan, M.I. Bichurin, Appl. Phys. Lett. 88, 183507 (2006)

    Article  ADS  Google Scholar 

  10. R. Bergs, R.A. Islam, M. Vickers, H. Stephanou, J. Appl. Phys. 101, 024108 (2007)

    Article  ADS  Google Scholar 

  11. Y. Chen, X.-Y. Zhang, C. Vittoria, V.G. Harris, Appl. Phys. Lett. 94, 102906 (2009)

    Article  ADS  Google Scholar 

  12. M. Vopsaroiu, J. Blackburn, M.G. Cain, Mater. Res. Soc. Symp. Proc. 1161, 574174 (2009)

    Google Scholar 

  13. M.I. Bichurin, I.A. Kornev, V.M. Petrov, A.S. Tatarenko, Yu.V. Kiliba, G. Srinivasan, Phys. Rev. B 64, 094409 (2001)

    Article  ADS  Google Scholar 

  14. J. Das, Y.Y. Song, N. Mo, P. Krivosik, C.E. Patton, Adv. Mater. 21, 2045 (2009)

    Article  Google Scholar 

  15. S.X. Dong, J. Zhai, J.F. Li, D. Viehland, Appl. Phys. Lett. 88, 082907 (2006)

    Article  ADS  Google Scholar 

  16. S. Shastry, G. Srinivasan, M.I. Bichurin, V.M. Petrov, A.S. Tatarenko, Phys. Rev. B 70, 064416 (2004)

    Article  ADS  Google Scholar 

  17. H. Béa, M. Gajek, M. Bibes, A. Barthélémy, J. Phys. Condens. Matter. 20, 434221 (2008)

    Article  Google Scholar 

  18. M. Gajek, M. Bibes, S. Fusil, K. Bouzehouane, J. Fontcuberta, A. Barthelemy, A. Fert, Nat. Mater. 6, 296 (2007)

    Article  ADS  Google Scholar 

  19. G. Srinivasan, E.T. Rasmussen, R. Hayes, Phys. Rev. B 67, 014418 (2003)

    Article  ADS  Google Scholar 

  20. Y.J. Wang, C.M. Leung, S.W. Or, X.Y. Zhao, H.S. Luo, X.K. Lv, Z.D. Zhang, Appl. Phys. A 97, 201 (2009)

    Article  ADS  Google Scholar 

  21. M. Liu, X. Li, H. Imrane, Y. Chen, T. Goodrich, K.S. Ziemer, J.Y. Huang, N.X. Sun, Appl. Phys. Lett. 90, 152501 (2007)

    Article  ADS  Google Scholar 

  22. Y. Chen, A.L. Geiler, T. Fitchorov, C. Vittoria, V.G. Harris, Appl. Phys. Lett. 95, 182501 (2009)

    Article  ADS  Google Scholar 

  23. K.E. Kamentsev, Y.K. Fetisov, G. Srinivasan, Tech. Phys. 52, 727 (2007)

    Article  Google Scholar 

  24. G. Srinivasan, R. Hayes, C.P. Devreugd, V.M. Laletsin, N. Paddubnaya, Appl. Phys. A 80, 891 (2005)

    Article  ADS  Google Scholar 

  25. P. Han, W. Yan, J. Tian, X. Huang, H. Pan, Appl. Phys. Lett. 86, 052902 (2005)

    Article  ADS  Google Scholar 

  26. Y.M. Jia, H.S. Luo, X.Y. Zhao, F.F. Wang, Adv. Mater. 20, 4776 (2008)

    Article  Google Scholar 

  27. S.B. Lang, H.L.W. Chan, Frontiers of Ferroelectricity (Springer, Berlin, 2007)

    Google Scholar 

  28. C.W. Nan, M.I. Bichurin, S. Dong, D. Viehland, J. Appl. Phys. 103, 031101 (2008)

    Article  ADS  Google Scholar 

  29. Y. Chen, T. Fitchorov, Z. Cai, K.S. Ziemer, C. Vittoria, V.G. Harris, J. Phys. D Appl. Phys. 43, 155001 (2010)

    Article  ADS  Google Scholar 

  30. C. Jullian, J.F. Li, D. Viehland, Appl. Phys. Lett. 83, 1196 (2003)

    Article  ADS  Google Scholar 

  31. X.J. Lou, J. Appl. Phys. 105, 024101 (2009)

    Article  ADS  Google Scholar 

  32. E.V. Colla, L.K. Chao, M.B. Weissman, D.D. Viehland, Phys. Rev. Lett. 85, 3033 (2000)

    Article  ADS  Google Scholar 

  33. Z.G. Ye, Y. Bing, J. Gao, A. Bokov, P. Stephens, B. Nohenda, G. Shirane, Phys. Rev. B 67, 104104 (2003)

    Article  ADS  Google Scholar 

  34. G. Xu, G. Shirane, J.R.D. Copley, P.M. Gehring, Phys. Rev. B 69, 064112 (2004)

    Article  ADS  Google Scholar 

  35. D. Viehland, J.F. Li, Philos. Mag. 84, 1969 (2004)

    Article  ADS  Google Scholar 

  36. E.V. Colla, P. Griffin, M. Delgado, M.B. Weissman, Phys. Rev. B 78, 054103 (2008)

    Article  ADS  Google Scholar 

  37. S.B. Majumder, Y.N. Mohapatra, D.C. Agrawal, Appl. Phys. Lett. 70, 138 (1997)

    Article  ADS  Google Scholar 

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Correspondence to Yajie Chen.

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Chen, Y., Fitchorov, T., Geiler, A.L. et al. Dynamic response of converse magnetoelectric effect in a PMN-PT-based multiferroic heterostructure. Appl. Phys. A 100, 1149–1155 (2010). https://doi.org/10.1007/s00339-010-5726-9

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  • DOI: https://doi.org/10.1007/s00339-010-5726-9

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