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Estimation of the Environmental Load of High- and Low-Density Polyethylene From South Korea Using a Mass Balance Approach

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Abstract

The accumulation of marine plastic debris is one of the main emerging environmental issues of the twenty first century. Numerous studies in recent decades have reported the level of plastic particles on the beaches and in oceans worldwide. However, it is still unclear how much plastic debris remains in the marine environment because the sampling methods for identifying and quantifying plastics from the environment have not been standardized; moreover, the methods are not guaranteed to find all of the plastics that do remain. The level of identified marine plastic debris may explain only the small portion of remaining plastics. To perform a quantitative estimation of remaining plastics, a mass balance analysis was performed for high- and low-density PE within the borders of South Korea during 1995–2012. Disposal methods such as incineration, land disposal, and recycling accounted for only approximately 40 % of PE use, whereas 60 % remained unaccounted for. The total unaccounted mass of high- and low-density PE to the marine environment during the evaluation period was 28 million tons. The corresponding contribution to marine plastic debris would be approximately 25,000 tons and 70 g km−2 of the world oceans assuming that the fraction entering the marine environment is 0.001 and that the degradation half-life is 50 years in seawater. Because the observed concentrations of plastics worldwide were much lower than the range expected by extrapolation from this mass balance study, it is considered that there probably is still a huge mass of unidentified plastic debris. Further research is therefore needed to fill this gap between the mass balance approximation and the identified marine plastics including a better estimation of the mass flux to the marine environment.

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References

  • Albertsson A (1980) The shape of the biodegradation curve for low and high density polyethenes in prolonged series of experiments. Eur Polym J 16:623–630

    Article  CAS  Google Scholar 

  • Andrady AL (2011) Microplastics in the marine environment. Mar Pollut Bull 62:1596–1605

    Article  CAS  Google Scholar 

  • Andrady AL, Neal MA (2009) Applications and societal benefits of plastic. Phil Trans R Soc B Biol Sci 364:1977–1984

    Article  CAS  Google Scholar 

  • Artham T, Sudhakar M, Venkatesan R, Madhavan Nair C, Murty K et al (2009) Biofouling and stability of synthetic polymers in sea water. Int Biodeterior Biodegrad 63:884–890

    Article  CAS  Google Scholar 

  • Barnes DKA, Galgani F, Thompson RC, Barlaz M (2009) Accumulation and fragmentation of the plastic debris in global environments. Phil Trans R Soc B Biol Sci 364:1985–1998

    Article  CAS  Google Scholar 

  • Cózar A, Echevarria F, González-Gordillo I, Irigoien X, Úbeda B, Hernández-León S et al (2014) Plastic debris in the open ocean. Proc Nat Acad Sci USA 111:10239–10244

    Article  Google Scholar 

  • Doyle MJ, Watson W, Bowlin NM, Sheavly SB (2011) Plastic particles in coastal pelagic ecosystems of the Northeast Pacific ocean. Mar Environ Res 71:41–52

    Article  CAS  Google Scholar 

  • Engler RE (2012) The complex interaction between marine debris and toxic chemicals in the ocean. Environ Sci Technol 46:12302–12315

    Article  CAS  Google Scholar 

  • Eriksen M, Maximenko N, Thiel M, Cummins A, Lattin G, Wilson S et al (2013) Plastic pollution in the South Pacific subtropical gyre. Mar Pollut Bull 68:71–76

    Article  CAS  Google Scholar 

  • Esmaeili A, Pourbabaee AA, Alikhani HA, Shabani F, Esmaeili E (2013) Biodegradation of low-density polyethylene (LDPE) mixed culture of Lysinibacillus xylanilyticus and Aspergillus niger in soil. PLoS One 8:e71720

    Article  CAS  Google Scholar 

  • Fletcher BL, Mackay ME (1996) A model of plastics recycling: does recycling reduce the amount of waste? Res Conserv Recycl 17:141–151

    Article  Google Scholar 

  • Goldstein MC, Rosenberg M, Cheng L (2012) Increased oceanic microplastic debris enhances oviposition in an endemic pelagic insect. Biol Lett 8:817–820

    Article  Google Scholar 

  • Harshvardhan K, Jha B (2013) Biodegradation of low-density polyethylene by marine bacteria from pelagic waters, Arabian Sea, India. Mar Pollut Bull 77:100–106

    Article  CAS  Google Scholar 

  • Hopewell J, Dvorak R, Kosior E (2009) Plastics recycling: challenges and opportunities. Phil Trans R Soc B Biol Sci 364:2115–2126

    Article  CAS  Google Scholar 

  • Horvat N, Ng FTT (1999) Tertiary polymer recycling: study of polyethylene thermolysis as a first step to synthetic diesel fuel. Fuel 78:459–470

    Article  CAS  Google Scholar 

  • Ivar do Sul JA, Costa MF (2014) The present and future of microplastic pollution in the marine environment. Environ Pollut 185:352–364

    Article  CAS  Google Scholar 

  • Jambeck JR, Geyer R, Wilcox C, Siegler TR, Perryman M, Andrady A et al (2015) Plastic waste inputs from land into the ocean. Science 347:768–771

    Article  CAS  Google Scholar 

  • Jang YC, Lee J, Hong S, Mok JY, Kim KS, Lee YJ et al (2014) Estimation of the annual flow and stock of marine debris in South Korea for management purposes. Mar Pollut Bull 86:505–511

    Article  CAS  Google Scholar 

  • Korea Ministry of Environment (2014) Status of the national waste generation and treatment (in Korean). Korea Ministry of Environment, SeJong City

    Google Scholar 

  • Law KL, Morét-Ferguson SE, Goodwin DS, Zettler ER, DeForce E, Kukulka T et al (2014) Distribution of surface plastic debris in the Eastern Pacific Ocean from an 11-year data set. Environ Sci Technol 48:4732–4738

    Article  CAS  Google Scholar 

  • Moore CJ (2008) Synthetic polymers in the marine environment: a rapidly increasing, long-term threat. Environ Res 108:131–139

    Article  CAS  Google Scholar 

  • Morét-Ferguson S, Law KL, Proskurowski G, Murphy EK, Peacock EE, Reddy CM (2010) The size, mass, and composition of plastic debris in the western North Atlantic Ocean. Mar Pollut Bull 60:1873–1878

    Article  Google Scholar 

  • Ng KL, Obbard JP (2006) Prevalence of microplastics in Singapore’s coastal marine environment. Mar Pollut Bull 52:761–767

    Article  CAS  Google Scholar 

  • Nowak B, Pajak J, Drozd-Bratkowicz M, Rymarz G (2011) Microorganisms participating in the biodegradation of modified polyethylene films in different soils under laboratory conditions. Int Biodeterior Biodegrad 45:49–55

    Google Scholar 

  • Orhan Y, Hrenovic J, Buyukgungor H (2004) Biodegradation of plastic compost bags under controlled soil conditions. Acta Chim Slov 51:579–588

    CAS  Google Scholar 

  • PlasticsEurope (2015) Plastics—the facts 2014/2015: an analysis of European plastics production, demand and waste data. Plastics Europe, Brussels, Belgium, p 34

  • Reisser J, Shaw J, Wilcox C, Hardesty BD, Proietti M, Thums M et al (2013) Marine plastic pollution in waters around Australia: characteristics, concentrations, and pathways. PLoS One 8:e80466

    Article  Google Scholar 

  • Restrepo-Flórez J-M, Bassi A, Thompson MR (2014) Microbial degradation and deterioration of polyethylene—a review. Int Biodet Biodeg 88:83–90

    Article  Google Scholar 

  • Sadri SS, Thompson RC (2014) On the quantity and composition of floating plastic debris entering and leaving the Tamar Estuary, Southwest England. Mar Pollut Bull 81:55–60

    Article  CAS  Google Scholar 

  • Statistics Korea (2014) Manufacturing industry trend analysis, 1995–2012 (in Korean). http://kosis.kr/. Accessed 23 July 2014

  • Storrier KL, McGlashan DJ, Bonellie S, Velander K (2007) Beach litter deposition at a selection of beaches in the Firth of Forth, Scotland. J Coast Res 23:813–822

    Article  Google Scholar 

  • United Nations Environment Programme (2011) UNEP year book 2011: emerging issues in our global environment. UNEP, Nairobi, p 79

    Google Scholar 

Download references

Acknowledgement

This research was supported by the National Research Foundation of Korea grant (Grant No. 2015R1A2A04003958).

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Correspondence to Jung-Hwan Kwon.

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Kim, M., Hyun, S. & Kwon, JH. Estimation of the Environmental Load of High- and Low-Density Polyethylene From South Korea Using a Mass Balance Approach. Arch Environ Contam Toxicol 69, 367–373 (2015). https://doi.org/10.1007/s00244-015-0192-1

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  • DOI: https://doi.org/10.1007/s00244-015-0192-1

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