Abstract
We have synthesized La2−x Sr x CuO4 thin films using atomic layer-by-layer molecular beam epitaxy (ALL-MBE). The films are high-quality—singe crystal, atomically smooth, and very homogeneous. The critical temperature (T c) shows a very little (<1 K) variation within a film of 10×10 mm 2 area. The large statistics (over 2000 films) is crucial to discern intrinsic properties. In these films, we have measured the absolute value of the magnetic penetration depth λ with the accuracy better than 1 % and mapped densely the entire overdoped side of the La2−x Sr x CuO4 phase diagram. A new scaling law is established accurately for the dependence of T c on the superfluid density. The scaling we observe is incompatible with the standard Bardeen-Cooper-Schrieffer picture and points to local pairing.
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Lee, P. A., Nagaosa, N., Wen, X. G.: Doping a Mott insulator: physics of high-temperature superconductivity. Rev. Mod. Phys. 78, 17–85 (2006)
Zaanen, J., Chakravarty, S., Senthil, T., Anderson, P. W., Lee, P., Schmalian, J., Imada, M., Pines, D., Randeria, M., Varma, C., Vojta, M., Rice, M.: Towards a complete theory of high Tc. Nature Phys. 2, 138–143 (2006)
Keimer, B., Kivelson, S. A., Norman, M. R., Uchida, S., Zaanen, J.: From quantum matter to high-temperature superconductivity in copper oxides. Nature 518, 179–186 (2015)
Uemura, Y. J., et al.: Universal correlations between Tc and ns/m* (carrier density over effective mass) in high- Tc cuprate superconductors. Phys. Rev. Lett. 62, 2317–2320 (1989)
Uemura, Y. J., et al.: Magnetic-field penetration depth in TI2Ba2CuO6 + δ in the overdoped regime. Nature 364, 605–607 (1993)
Niedermayer, C., et al.: Muon spin rotation study of the correlation between Tc and ns/m* in overdoped Tl2Ba2CuO6 + δ . Phys. Rev. Lett. 71, 1764–1767 (1993)
Bernhard, C., et al.: Magnetic penetration depth and condensate density of cuprate high- Tc superconductors determined by muon-spin-rotation experiments. Phys. Rev. B 52, 10488–10498 (1995)
Panagopoulos, C., et al.: Superfluid response in monolayer high- Tc cuprates. Phys. Rev. B 67, 220502 (2003)
Tallon, J. L., Loram, J. W., Cooper, J. R., Panagopoulos, C., Bernhard, C.: Superfluid density in cuprate high- Tc superconductors: a new paradigm. Phys. Rev. B 68, 180501 (2003)
Bozovic, I.: Atomic-layer engineering of superconducting oxides: yesterday, today, tomorrow. IEEE Trans. Appl. Supercond. 11, 2686–2695 (2001)
Gozar, A., et al.: Interface superconductivity between a metal and a Mott insulator. Nature 455, 782–785 (2008)
Logvenov, G., Gozar, A., Bozovic, I.: High-temperature superconductivity in a single copper-oxygen plane. Science 326, 699–702 (2009)
Hebard, A. F., Fiory, A. T.: Evidence for the Kosterlitz-Thouless transition in thin superconducting aluminum films. Phys. Rev. Lett. 44, 291–294 (1980)
Claassen, J. H., Reeves, M. E., Soulen, Jr R.J: A contactless method for measurement of the critical current density and critical temperature of superconducting rings. Rev. Sci. Instrum. 62, 996–1004 (1991)
Clem, J. R., Coffey, M. W.: Vortex dynamics in a type-II superconducting film and complex linear-response functions. Phys. Rev. B 46, 14662–14674 (1992)
Turneaure, S. J., Ulm, E. R., Lemberger, T. R.: Numerical modeling of a two-coil apparatus for measuring the magnetic penetration depth in superconducting films and arrays. J. Appl. Phys. 79, 4221–4227 (1996)
Locquet, J. P., et al.: Variation of the in-plane penetration depth λ ab as a function of doping in La2−xSrxCuO4 + δ thin films on SrTiO3: implications for the overdoped state. Phys. Rev. B 54, 7481–7488 (1996)
Turneaure, S. J., Pesetski, A. A., Lemberger, T. R.: Numerical modeling and experimental considerations for a two-coil apparatus to measure the complex conductivity of superconducting films. J. Appl. Phys. 83, 4334–4343 (1998)
Lemberger, T. R., et al.: Superconductor-to-metal quantum phase transition in overdoped La2−xSrxCuO4. Phys. Rev. B 83, 140507 (2011)
Božović, I., He, X., Wu, J., Bollinger, A. T.: Dependence of critical temperature in overdoped copper oxides on superfluid density. Nature 536, 309–311 (2016)
Hirschfeld, P. J., Goldenfeld, N.: Effect of strong scattering on the low-temperature penetration depth of a d-wave superconductor. Phys. Rev. B 48, 4219–4222 (1993)
Hosseini, A., et al.: Microwave spectroscopy of thermally excited quasi-particles in YBa2Cu3O6.99. Phys. Rev. B 60, 1349–1359 (1999)
Broun, D. M., et al.: Superfluid density in a highly underdoped YBa2Cu3O6+y superconductor. Phys. Rev. Lett. 99, 237003 (2007)
Zaanen, J.: Superconducting electrons go missing. Nature 536, 282–283 (2016)
Kivelson, S. A.: On the character of the superconductor to metal transition in overdoped cuprates. Journal Club for Condensed Matter Physics, 18 (2016)
Leggett, A.: Quantum Liquids. Oxford University Press (2006). chapters 3.3 and 3.4
Leggett, A.: On the superfluid fraction of an arbitrary many-body system at T = 0. J. Stat. Phys. 93, 927 (1998)
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This research was done at the Brookhaven National Laboratory and was supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. X.H. is supported by the Gordon and Betty Moore Foundation’s EPiQS Initiative through Grant GBMF4410.
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Božović, I., He, X., Wu, J. et al. The Demise of Superfluid Density in Overdoped La2−x Sr x CuO4 Films Grown by Molecular Beam Epitaxy. J Supercond Nov Magn 30, 1345–1348 (2017). https://doi.org/10.1007/s10948-016-3819-1
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DOI: https://doi.org/10.1007/s10948-016-3819-1