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The Demise of Superfluid Density in Overdoped La2−x Sr x CuO4 Films Grown by Molecular Beam Epitaxy

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Abstract

We have synthesized La2−x Sr x CuO4 thin films using atomic layer-by-layer molecular beam epitaxy (ALL-MBE). The films are high-quality—singe crystal, atomically smooth, and very homogeneous. The critical temperature (T c) shows a very little (<1 K) variation within a film of 10×10 mm 2 area. The large statistics (over 2000 films) is crucial to discern intrinsic properties. In these films, we have measured the absolute value of the magnetic penetration depth λ with the accuracy better than 1 % and mapped densely the entire overdoped side of the La2−x Sr x CuO4 phase diagram. A new scaling law is established accurately for the dependence of T c on the superfluid density. The scaling we observe is incompatible with the standard Bardeen-Cooper-Schrieffer picture and points to local pairing.

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References

  1. Lee, P. A., Nagaosa, N., Wen, X. G.: Doping a Mott insulator: physics of high-temperature superconductivity. Rev. Mod. Phys. 78, 17–85 (2006)

    Article  ADS  Google Scholar 

  2. Zaanen, J., Chakravarty, S., Senthil, T., Anderson, P. W., Lee, P., Schmalian, J., Imada, M., Pines, D., Randeria, M., Varma, C., Vojta, M., Rice, M.: Towards a complete theory of high Tc. Nature Phys. 2, 138–143 (2006)

    Article  Google Scholar 

  3. Keimer, B., Kivelson, S. A., Norman, M. R., Uchida, S., Zaanen, J.: From quantum matter to high-temperature superconductivity in copper oxides. Nature 518, 179–186 (2015)

    Article  ADS  Google Scholar 

  4. Uemura, Y. J., et al.: Universal correlations between Tc and ns/m* (carrier density over effective mass) in high- Tc cuprate superconductors. Phys. Rev. Lett. 62, 2317–2320 (1989)

    Article  ADS  Google Scholar 

  5. Uemura, Y. J., et al.: Magnetic-field penetration depth in TI2Ba2CuO6 + δ in the overdoped regime. Nature 364, 605–607 (1993)

    Article  ADS  Google Scholar 

  6. Niedermayer, C., et al.: Muon spin rotation study of the correlation between Tc and ns/m* in overdoped Tl2Ba2CuO6 + δ . Phys. Rev. Lett. 71, 1764–1767 (1993)

    Article  ADS  Google Scholar 

  7. Bernhard, C., et al.: Magnetic penetration depth and condensate density of cuprate high- Tc superconductors determined by muon-spin-rotation experiments. Phys. Rev. B 52, 10488–10498 (1995)

    Article  ADS  Google Scholar 

  8. Panagopoulos, C., et al.: Superfluid response in monolayer high- Tc cuprates. Phys. Rev. B 67, 220502 (2003)

    Article  ADS  Google Scholar 

  9. Tallon, J. L., Loram, J. W., Cooper, J. R., Panagopoulos, C., Bernhard, C.: Superfluid density in cuprate high- Tc superconductors: a new paradigm. Phys. Rev. B 68, 180501 (2003)

    Article  ADS  Google Scholar 

  10. Bozovic, I.: Atomic-layer engineering of superconducting oxides: yesterday, today, tomorrow. IEEE Trans. Appl. Supercond. 11, 2686–2695 (2001)

    Article  Google Scholar 

  11. Gozar, A., et al.: Interface superconductivity between a metal and a Mott insulator. Nature 455, 782–785 (2008)

    Article  ADS  Google Scholar 

  12. Logvenov, G., Gozar, A., Bozovic, I.: High-temperature superconductivity in a single copper-oxygen plane. Science 326, 699–702 (2009)

    Article  ADS  Google Scholar 

  13. Hebard, A. F., Fiory, A. T.: Evidence for the Kosterlitz-Thouless transition in thin superconducting aluminum films. Phys. Rev. Lett. 44, 291–294 (1980)

    Article  ADS  Google Scholar 

  14. Claassen, J. H., Reeves, M. E., Soulen, Jr R.J: A contactless method for measurement of the critical current density and critical temperature of superconducting rings. Rev. Sci. Instrum. 62, 996–1004 (1991)

    Article  ADS  Google Scholar 

  15. Clem, J. R., Coffey, M. W.: Vortex dynamics in a type-II superconducting film and complex linear-response functions. Phys. Rev. B 46, 14662–14674 (1992)

    Article  ADS  Google Scholar 

  16. Turneaure, S. J., Ulm, E. R., Lemberger, T. R.: Numerical modeling of a two-coil apparatus for measuring the magnetic penetration depth in superconducting films and arrays. J. Appl. Phys. 79, 4221–4227 (1996)

    Article  ADS  Google Scholar 

  17. Locquet, J. P., et al.: Variation of the in-plane penetration depth λ ab as a function of doping in La2−xSrxCuO4 + δ thin films on SrTiO3: implications for the overdoped state. Phys. Rev. B 54, 7481–7488 (1996)

    Article  ADS  Google Scholar 

  18. Turneaure, S. J., Pesetski, A. A., Lemberger, T. R.: Numerical modeling and experimental considerations for a two-coil apparatus to measure the complex conductivity of superconducting films. J. Appl. Phys. 83, 4334–4343 (1998)

    Article  ADS  Google Scholar 

  19. Lemberger, T. R., et al.: Superconductor-to-metal quantum phase transition in overdoped La2−xSrxCuO4. Phys. Rev. B 83, 140507 (2011)

    Article  ADS  Google Scholar 

  20. Božović, I., He, X., Wu, J., Bollinger, A. T.: Dependence of critical temperature in overdoped copper oxides on superfluid density. Nature 536, 309–311 (2016)

    Article  ADS  Google Scholar 

  21. Hirschfeld, P. J., Goldenfeld, N.: Effect of strong scattering on the low-temperature penetration depth of a d-wave superconductor. Phys. Rev. B 48, 4219–4222 (1993)

    Article  ADS  Google Scholar 

  22. Hosseini, A., et al.: Microwave spectroscopy of thermally excited quasi-particles in YBa2Cu3O6.99. Phys. Rev. B 60, 1349–1359 (1999)

    Article  ADS  Google Scholar 

  23. Broun, D. M., et al.: Superfluid density in a highly underdoped YBa2Cu3O6+y superconductor. Phys. Rev. Lett. 99, 237003 (2007)

    Article  ADS  Google Scholar 

  24. Zaanen, J.: Superconducting electrons go missing. Nature 536, 282–283 (2016)

    Article  ADS  Google Scholar 

  25. Kivelson, S. A.: On the character of the superconductor to metal transition in overdoped cuprates. Journal Club for Condensed Matter Physics, 18 (2016)

  26. Leggett, A.: Quantum Liquids. Oxford University Press (2006). chapters 3.3 and 3.4

  27. Leggett, A.: On the superfluid fraction of an arbitrary many-body system at T = 0. J. Stat. Phys. 93, 927 (1998)

    Article  ADS  MathSciNet  MATH  Google Scholar 

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Acknowledgments

This research was done at the Brookhaven National Laboratory and was supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. X.H. is supported by the Gordon and Betty Moore Foundation’s EPiQS Initiative through Grant GBMF4410.

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Božović, I., He, X., Wu, J. et al. The Demise of Superfluid Density in Overdoped La2−x Sr x CuO4 Films Grown by Molecular Beam Epitaxy. J Supercond Nov Magn 30, 1345–1348 (2017). https://doi.org/10.1007/s10948-016-3819-1

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  • DOI: https://doi.org/10.1007/s10948-016-3819-1

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