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Deposition–Precipitation and Stabilization of a Silica-Supported Au Catalyst by Surface Modification with Carbon Nitride

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Abstract

A silica support is modified by carbon nitride in order to allow for the deposition–precipitation of Au, which is normally unfavorable. The resulting catalyst is highly stable even after the removal of the carbon nitride layer at high temperature and shows good catalytic activity for the oxidation of CO in air.

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References

  1. Ma Z, Dai S (2011) Acs Catal 1:805–818

    Article  CAS  Google Scholar 

  2. Hutchings GJ, Haruta M (2005) Appl Catal A 291:2–5

    Article  CAS  Google Scholar 

  3. Haruta M (2002) Cattech 6:102–115

    Article  CAS  Google Scholar 

  4. Thompson DT, Bond GC (1999) Catal Rev 41:319–388

    Article  Google Scholar 

  5. Lee B, Ma Z, Zhang ZT, Park C, Dai S (2009) Micropor Mesopor Mater 122:160–167

    Article  CAS  Google Scholar 

  6. Wolf A, Schuth F (2002) Appl Catal a-Gen 226:1–13

    Article  CAS  Google Scholar 

  7. Haruta M (1997) Catal Today 36:153–166

    Article  CAS  Google Scholar 

  8. Al-Sayari S, Carley AF, Taylor SH, Hutchings GJ (2007) Top Catal 44:123–128

    Article  CAS  Google Scholar 

  9. Carabineiro SAC, Silva AMT, Drazic G, Tavares PB, Figueiredo JL (2010) Catal Today 154:293–302

    Article  CAS  Google Scholar 

  10. Comotti M, Li WC, Spliethoff B, Schuth F (2006) J Am Chem Soc 128:917–924

    Article  CAS  Google Scholar 

  11. Yan WF, Mahurin SM, Chen B, Overbury SH, Dai S (2005) J Phys Chem B 109:15489–15496

    Article  CAS  Google Scholar 

  12. Ma Z, Dai S (2011) Nano Res 4:3–32

    Article  CAS  Google Scholar 

  13. Bore MT, Mokhonoana MP, Ward TL, Coville NJ, Datye AK (2006) Micropor Mesopor Mater 95:118–125

    Article  CAS  Google Scholar 

  14. Qian K, Huang WX, Fang J, Lv SS, He B, Jiang ZQ, Wei SQ (2008) J Catal 255:269–278

    Article  CAS  Google Scholar 

  15. Qian K, Lv SS, Xiao XY, Sun HX, Lu JQ, Luo MF, Huang WX (2009) J Mol Catal a-Chem 306:40–47

    Article  CAS  Google Scholar 

  16. Zhu HG, Liang CD, Yan WF, Overbury SH, Dai S (2006) J Phys Chem B 110:10842–10848

    Article  CAS  Google Scholar 

  17. Kawaguchi M, Nozaki K (1995) Chem Mater 7:257–264

    Article  CAS  Google Scholar 

  18. Wang Y, Wang XC, Antonietti M (2012) Angew Chem Int Edit 51:68–89

    Article  CAS  Google Scholar 

  19. Somodi F, Borbath I, Hegedus M, Tompos A, Sajo IE, Szegedi A, Rojas S, Fierro JLG, Margitfalvi JL (2008) Appl Catal a-Gen 347:216–222

    Article  CAS  Google Scholar 

  20. Ghosh A, Patra CR, Mukherjee P, Sastry M, Kumar R (2003) Micropor Mesopor Mater 58:201–211

    Article  CAS  Google Scholar 

  21. Yang CM, Liu PH, Ho YF, Chiu CY, Chao KJ (2003) Chem Mater 15:275–280

    Article  CAS  Google Scholar 

  22. Wang Y, Yao J, Li HR, Su DS, Antonietti M (2011) J Am Chem Soc 133:2362–2365

    Article  CAS  Google Scholar 

  23. Liu JH, Zhang TK, Wang ZC, Dawson G, Chen W (2011) J Mater Chem 21:14398–14401

    Article  CAS  Google Scholar 

  24. Zhang JA, Li YA, Zhu PW, Huang DH, Wu S, Cui QL, Zou GT (2011) Diam Relat Mater 20:385–388

    Article  Google Scholar 

  25. Miller DR, Wang JJ, Gillan EG (2002) J Mater Chem 12:2463–2469

    Article  CAS  Google Scholar 

  26. Meng YL, Xin G, Chen D (2011) Optoelectron Adv Mater 5:648–650

    CAS  Google Scholar 

  27. Zhang JS, Chen XF, Takanabe K, Maeda K, Domen K, Epping JD, Fu XZ, Antonietti M, Wang XC (2010) Angew Chem Int Edit 49:441–444

    Article  CAS  Google Scholar 

  28. Kim TW, Chung PW, Lin VSY (2010) Chem Mater 22:5093–5104

    Article  CAS  Google Scholar 

  29. Liu R, Mahurin SM, Li C, Unocic RR, Idrobo JC, Gao HJ, Pennycook SJ, Dai S (2011) Angew Chem Int Edit 50:6799–6802

    Article  CAS  Google Scholar 

  30. Li XF, Zhang J, Shen LH, Ma YM, Lei WW, Cui QL, Zou GT (2009) Appl Phys A 94:387–392

    Article  CAS  Google Scholar 

  31. Guo QX, Yang Q, Yi CQ, Zhu L, Xie Y (2005) Carbon 43:1386–1391

    Article  CAS  Google Scholar 

  32. Komatsu T, Nakamura T (2001) J Mater Chem 11:474–478

    Article  CAS  Google Scholar 

  33. Zhu JJ, Carabineiro SAC, Shan D, Faria JL, Zhu YJ, Figueiredo JL (2010) J Catal 274:207–214

    Article  CAS  Google Scholar 

  34. Singh JA, Overbury SH, Dudney NJ, Li MJ, Veith GM (2012) Acs Catal 2:1138–1146

    Article  CAS  Google Scholar 

  35. Veith GM, Lupini AR, Rashkeev S, Pennycook SJ, Mullins DR, Schwartz V, Bridges CA, Dudney NJ (2009) J Catal 262:92–101

    Article  CAS  Google Scholar 

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Acknowledgments

The research was sponsored by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, US Department of Energy, under contract no. DE-AC05-00OR22725 with Oak Ridge National Laboratory managed and operated by UT-Battelle, LLC.

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Authors and Affiliations

  1. Department of Chemistry, University of Tennessee, Knoxville, TN, 37996-1600, USA

    Andrew J. Binder & Sheng Dai

  2. Chemical Sciences Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37831, USA

    Zhen-An Qiao & Sheng Dai

  3. Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37831, USA

    Gabriel M. Veith

Authors
  1. Andrew J. Binder
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  2. Zhen-An Qiao
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  3. Gabriel M. Veith
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  4. Sheng Dai
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Corresponding author

Correspondence to Sheng Dai.

Electronic supplementary material

Below is the link to the electronic supplementary material.

10562_2013_1093_MOESM1_ESM.docx

XRD data and TEM images comparing the Au/CN/SBA-15 sample after hydrogen reduction and after catalytic testing, as well as further catalytic tests on Au/CN/SBA-15 can be found in supporting information (DOCX 1164 kb)

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Binder, A.J., Qiao, ZA., Veith, G.M. et al. Deposition–Precipitation and Stabilization of a Silica-Supported Au Catalyst by Surface Modification with Carbon Nitride. Catal Lett 143, 1339–1345 (2013). https://doi.org/10.1007/s10562-013-1093-4

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  • DOI: https://doi.org/10.1007/s10562-013-1093-4

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