Skip to main content
Log in

Angle-dependent electron energy spectra resulting from autoionizing Ne⋆ (3s 3 P 2) +H(12 S) collisions

  • Published:
Zeitschrift für Physik D Atoms, Molecules and Clusters

Abstract

Experimental angle-dependent electron energy spectra for the autoionization complex Ne*(3s 3 P 2)+H(12 S), leading to Penning and associative ionization, are reported. The data, measured at thermal collision energies (Ē rel∼51 meV), clearly show an angular variation of the spectral shape, indicating that electrons with angular momentuml>0 participate in the autoionization process. The corresponding non-isotropic electron emission leads to a correlation between the impact parameter-dependent heavy-particle dynamics and the observed electron energy spectrum at a certain detection angle. The experimental results are qualitatively discussed in connection with previous work on the system He*(23 S)+H(12 S). Furthermore, we present quantum mechanical model-calculations for the electron energy spectrum on the basis of available potential data.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  1. Ruf, M.-W., Yencha, A.J., Hotop, H.: Z. Phys. D5, 9 (1987)

    Google Scholar 

  2. Müller, M.W., Bussert, W., Ruf, M.-W., Hotop, H., Meyer, W.: Phys. Rev. Lett.59, 2279 (1987)

    Google Scholar 

  3. Waibel, H., Ruf, M.-W., Hotop, H.: Z. Phys. D9, 191 (1988)

    Google Scholar 

  4. Mitsuke, K., Kusafuka, K., Ohno, K.: J. Phys. Chem.93, 3062 (1989)

    Google Scholar 

  5. Merz, A., Müller, M.W., Ruf, M.-W., Hotop, H., Meyer, W., Movre, M.: Chem. Phys. Lett.160, 377 (1989)

    Google Scholar 

  6. Merz, A., Müller, M.W., Ruf, M.-W., Hotop, H., Meyer, W., Movre, M.: Chem. Phys.145, 219 (1990)

    Google Scholar 

  7. Hotop, H., Ruf, M.-W., Yencha, A.J., Fricke, B.: Ann. Phys. (Leipzig)47, 635 (1990)

    Google Scholar 

  8. Khan, A., Siddiqui, H.R., Siska, P.E.: J. Chem. Phys.95, 3371 (1991)

    Google Scholar 

  9. Ohno, K., Takami, T., Mitsuke, K.: J. Chem. Phys.94, 2675 (1991)

    Google Scholar 

  10. Merz, A., Ruf, M.-W., Hotop, H.: Phys. Rev. Lett.69, 3467 (1992)

    Google Scholar 

  11. Bardou, F., Emile, O., Courty, J.-M., Westbrook, C.I., Aspect, A.: Europhys. Lett.20, 681 (1992)

    Google Scholar 

  12. Longley, E.J., Dunlavy, D.C., Falcetta, M.F., Bevsek, H.M., Siska, P.E.: J. Phys. Chem.97, 2097 (1993)

    Google Scholar 

  13. Merz, A., Ruf, M.-W., Hotop, H., Movre, M., Meyer, W.: In: AIPConference Proceedings 295. The physics of electronic and atomic collisions, XVIII ICPEAC. Aarhus, Denmark, 1993 Andersen, T., Fastrup, B., Folkmann, F., Knudsen, H., Andersen, N. (eds.), p. 852. New York: American Institute of Physics 1993

    Google Scholar 

  14. Rutherford, G.H., Soletzky, P.A., Bryan, W.H., Dunning, F.B., Walters, G.K.: Phys. Rev. A46, 230 (1992)

    Google Scholar 

  15. Padial, N.T., Cohen, J.S., Martin, R.L., Lane, N.F.: Phys. Rev. A40, 117 (1989)

    Google Scholar 

  16. Müller, M.W., Merz, A., Ruf, M.-W., Hotop, H., Meyer, W., Movre, M.: Z. Phys. D21, 89 (1991)

    Google Scholar 

  17. Ishida, T.: Chem. Phys. Lett.211, 1 (1993)

    Google Scholar 

  18. Sarpal, B.: J. Phys. B26, 4145 (1993)

    Google Scholar 

  19. Movre, M., Meyer, W.: J. Chem. Phys. (submitted for publication)

  20. Movre, M., Meyer, W., Merz, A., Ruf, M.-W., Hotop, H.: Chem. Phys. Lett. (submitted for publication)

  21. Aguilar, A., Brunetti, B., Gonzalez, M., Vecchiocattivi, F.: Chem. Phys.145, 211 (1990)

    Google Scholar 

  22. Aguilar-Navarro, A., Brunetti, B., Falcinelli, S., Gonzalez, M., Vecchiocattivi, F.: J. Chem. Phys.96, 433 (1992)

    Google Scholar 

  23. Schohl, S., Müller, M.W., Meijer, H.A.J., Ruf, M.-W., Hotop, H., Morgner, H.: Z. Phys. D16, 237 (1990)

    Google Scholar 

  24. Khan, A., Siddiqui, H.R., Siska, P.E.: J. Chem. Phys.94, 2588 (1991)

    Google Scholar 

  25. Baudon, J., Feron, P., Miniatura, C., Perales, F., Reinhardt, J., Robert, J., Haberland, H., Brunetti, B., Vecchiocattivi, F.: J. Chem. Phys.95, 1801 (1991)

    Google Scholar 

  26. Lorenzen, J., Hotop, H., Ruf, M.-W., Morgner, H.: Z. Phys. A297, 19 (1980)

    Google Scholar 

  27. Lorenzen, J., Morgner, H., Bußert, W., Ruf, M.-W., Hotop, H.: Z. Phys. A310, 141 (1983)

    Google Scholar 

  28. Niehaus, A.: Phys. Rep.186, 149 (1990)

    Google Scholar 

  29. Morgner, H.: J. Phys. B12, 2171 (1979)

    Google Scholar 

  30. Hickman, A.P., Morgner, H.: J. Phys. B9, 1765 (1976)

    Google Scholar 

  31. Ebding, T., Niehaus, A.: Z. Phys.270, 43 (1974)

    Google Scholar 

  32. Morgner, H., Niehaus, A.: J. Phys. B12, 1805 (1979)

    Google Scholar 

  33. Merz, A., Ruf, M.-W., Hotop, H., Movre, M., Meyer, W.: J. Phys. B (accepted for publication)

  34. Schohl, S., Klar, D., Kraft, T., Meijer, H.A.J., Ruf, M.-W., Schmitz, U., Smith, S.J., Hotop, H.: Z. Phys. D21, 25 (1991)

    Google Scholar 

  35. Miller, W.H.: J. Chem. Phys.52, 3563 (1970)

    Google Scholar 

  36. Niehaus, A.: Adv. Chem. Phys.45, 399 (1981)

    Google Scholar 

  37. Micha, D.A., Nakamura, H.: Phys. Rev. A11, 1988 (1975)

    Google Scholar 

  38. Rosmus, P., Reinsch, E.-A.: Z. Naturforsch.35a, 1066 (1980)

    Google Scholar 

  39. Gianturco, F.A., Niedner, G., Noll, M., Semprini, E., Stefani, F., Toennies, J.P.: Z. Phys. D7, 281 (1987)

    Google Scholar 

  40. Zemke, W.T., Olson, R.E., Verma, K.K., Stwalley, W.C., Liu, B.: J. Chem. Phys.80, 356 (1984)

    Google Scholar 

  41. Siska, P.E.: (private communication)

  42. Bieniek, R.J.: Phys. Rev. A18, 392 (1978)

    Google Scholar 

  43. Siska, P.E.: Rev. Mod. Phys.65, 2 (1993)

    Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Rights and permissions

Reprints and permissions

About this article

Cite this article

Merz, A., Ruf, M.W. & Hotop, H. Angle-dependent electron energy spectra resulting from autoionizing Ne⋆ (3s 3 P 2) +H(12 S) collisions. Z Phys D - Atoms, Molecules and Clusters 32, 197–203 (1994). https://doi.org/10.1007/BF01437148

Download citation

  • Received:

  • Revised:

  • Issue Date:

  • DOI: https://doi.org/10.1007/BF01437148

PACS

Navigation