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Absence of tetramethylene diradical intermediates in Lewis acid catalyzed group transfer polymerization

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Summary

A diradical tetramethylene intermediate in Lewis acid catalyzed Group Transfer Polymerization of methyl acrylate is unlikely based on the lack of incorporation of styrene during methyl acrylate polymerizations.

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References

  1. R. Hertler, D. Y. Sogah, O. W. Webster, B. M. Trost, Macromolecules (1984) 17, 1415.

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  2. O. W. Webster, Group Transfer Polymerization, Encyclopedia of Polymer Science and Engineering. Vol. 7. (1987) p. 580.

  3. H. K. Hall, Jr., Angew. Chem. Int. Ed. Eng. (1983) 22, 440.

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Authors and Affiliations

  1. C.S. Marvel Laboratories, Department of Chemistry, University of Arizona, 85721, Tucson, AZ, USA

    Hester A. Clever & H. K. Hall Jr.

Authors
  1. Hester A. Clever
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  2. H. K. Hall Jr.
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Clever, H.A., Hall, H.K. Absence of tetramethylene diradical intermediates in Lewis acid catalyzed group transfer polymerization. Polymer Bulletin 21, 179–182 (1989). https://doi.org/10.1007/BF00266170

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  • DOI: https://doi.org/10.1007/BF00266170

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