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Polymerization of Nonfood Biomass-Derived Monomers to Sustainable Polymers

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Book cover Selective Catalysis for Renewable Feedstocks and Chemicals

Part of the book series: Topics in Current Chemistry ((TOPCURRCHEM,volume 353))

Abstract

The development of sustainable routes to fine chemicals, liquid fuels, and polymeric materials from natural resources has attracted significant attention from academia, industry, the general public, and governments owing to dwindling fossil resources, surging energy demand, global warming concerns, and other environmental problems. Cellulosic material, such as grasses, trees, corn stover, or wheat straw, is the most abundant nonfood renewable biomass resources on earth. Such annually renewable material can potentially meet our future needs with a low carbon footprint if it can be efficiently converted into fuels, value added chemicals, or polymeric materials. This chapter focuses on various renewable monomers derived directly from cellulose or cellulose platforms and corresponding sustainable polymers or copolymers produced therefrom. Recent advances related to the polymerization processes and the properties of novel biomass-derived polymers are also reviewed and discussed.

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Abbreviations

β MMBL:

β-Methyl-α-methylene-γ-butyrolactone

γ MMBL:

γ-Methyl-α-methylene-γ-butyrolactone

ATRP:

Atom transfer radical polymerization

nBA:

n-Butyl acrylate

BM:

Bismaleimide

CGC:

Me2Si(η 5-(Me4C5)(tBuN)

CL:

Caprolactone

CLP:

Classical Lewis pair

Cp:

η 5-Cyclopentadienyl

DA:

Diels–Alder

DIOP:

Diisooctyl phthalate

DMAP:

4-Dimethylaminopyridine

DMF:

N,N-Dimethylformamide

DOE:

Department of energy

EBDMI:

C2H4(η 5-4,7-dimethylindenyl)2

EBI:

C2H4(η 5-indenyl)2

FLP:

Frustrated Lewis pair

Flu:

η 5- or η 3-Fluorenyl

FA:

Furfuryl alcohol

FMA:

Furfuryl methacrylate

GHG:

Greenhouse gas

GPC:

Gel permeation chromatography

GTP:

Group transfer polymerization

HMF:

5-Hydroxymethylfurfural

ItBu:

1,3-Di-tert-butylimidazol-2-ylidene

ICD:

β-Isocupreidine

ICD:

β-Isocupreidine

IMes:

1,3-Bis(2,4,6-trimethylphenyl)imidazol-2-ylidene

it:

Isotactic (mm)

LA:

Lactic acid or lactide

LPP:

Lewis pair polymerization

MBL:

α-Methylene-γ-butyrolactone

MEP:

1,8-Bis(maleimido)-1-ethylpropane

MIMA:

Maleimide methacrylate

MMA:

Methyl methacrylate

M n (M w):

Number (weight) average molecular weight

MW:

Molecular weight

MWD:

Molecular weight distribution

NHC:

N-Heterocyclic carbene

OSA:

Oligo(isosorbide adipate)

OSS:

Oligo(isosorbide suberate)

PASA:

Poly(aspartic acid)

PDI:

Polydispersity index

PET:

Poly(ethylene terephthalate)

PFS:

Poly(2,5-furandimethylene succinate)

PGA:

Poly(glutamic acid)

PHBHV:

Bis-hydroxylated poly(3-hydroxybutyrate-co-3-hydroxyvalerate) oligomers

PHUs:

Polyhydroxyurethanes

PLA:

Polylactide

PMMA:

Poly(methyl methacrylate)

PP:

Polypropylene

REM:

Rare earth metal

ROP:

Ring-opening polymerization

RSKA:

Trialkylsilyl methyl dimethylketene acetal

RT:

Room temperature

st:

Syndiotactic (rr)

SA:

Succinic acid

SDH:

Isosorbide dihexanoate

SEM:

Scanning electron microscopy

T g :

Glass transition temperature

THF:

Tetrahydrofuran

TOF:

Turnover frequency

TPT:

1,3,4-Triphenyl-4,5-dihydro-1H-1,2,4-triazol-5-ylidene

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Acknowledgments

This work was supported by the 1,000 Talents Young program and National Natural Science Foundation of China (NSFC) program (grant #21374040 to Y. Zhang) and by the US Department of Energy-Office of Basic Energy Sciences, grant DE-FG02-10ER16193 (to E. Y.-X. Chen).

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  1. State Key Laboratory of Supramolecular Structure and Materials, College of Chemistry, Jilin University, 2699 Qianjin Street, Changchun, Jilin, 130012, People’s Republic of China

    Yuetao Zhang

  2. Department of Chemistry, Colorado State University, Fort Collins, CO, 80523-1872, USA

    Yuetao Zhang & Eugene Y-X Chen

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  1. Department of Chemistry and Biochemistry, University of Oklahoma, Norman, Oklahoma, USA

    Kenneth M. Nicholas

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Zhang, Y., Chen, E.YX. (2014). Polymerization of Nonfood Biomass-Derived Monomers to Sustainable Polymers. In: Nicholas, K. (eds) Selective Catalysis for Renewable Feedstocks and Chemicals. Topics in Current Chemistry, vol 353. Springer, Cham. https://doi.org/10.1007/128_2014_539

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